Publications

We have used a deep-depletion CCD camera in single-hit mode to measure X-ray conversion efficiencies with Z-Beamlet and Z-Petawatt. Z-Petawatt is superior to Z-Beamlet for X-rays harder than 10 keV. For diffraction samples with Z > 42, we likely require X-rays with 15 keV or higher photon energy (Z-Petawatt). We are developing a robust, reproducible setup for X-ray polycapillaries as a part for X-ray diffraction experiments (XRD).

Helium or neopentane can be used as surrogate gas fill for deuterium (D2) or deuterium-tritium (DT) in laser-plasma interaction studies. Surrogates are convenient to avoid flammability hazards or the integration of cryogenics in an experiment. To test the degree of equivalency between deuterium and helium, experiments were conducted in the Pecos target chamber at Sandia National Laboratories. Observables such as laser propagation and signatures of laser-plasma instabilities (LPI) were recorded for multiple laser and target configurations. It was found that some observables can differ significantly despite the apparent similarity of the gases with respect to molecular charge and weight. While a qualitative behaviour of the interaction may very well be studied by finding a suitable compromise of laser absorption, electron density, and LPI cross sections, a quantitative investigation of expected values for deuterium fills at high laser intensities is not likely to succeed with surrogate gases.

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Diagnostics in high energy density physics, shock physics, and related fields are primarily driven by a need to record rapidly time-evolving signals in single-shot events. These measurements are often limited by channel count and signal degradation issues on cable links between the detector and digitizer. We present the Ultrafast Pixel Array Camera (UPAC), a compact and flexible detector readout system with 32 waveform-recording channels at up to 10 Gsample/s and 1.8 GHz analog bandwidth. The compact footprint allows the UPAC to be directly embedded in the detector environment. A key enabling technology is the PSEC4A chip, an eight-channel switch-capacitor array sampling device with up to 1056 samples/channel. The UPAC system includes a high-density input connector that can plug directly into an application-specific detector board, programmable control, and serial readout, with less than 5 W of power consumption in full operation. We present the UPAC design and characterization, including a measured timing resolution of ∼20 ps or better on acquisitions of sub-nanosecond pulses with minimal system calibrations. Example applications of the UPAC are also shown to demonstrate operation of a solid-state streak camera, an ultrafast imaging array, and a neutron time-of-flight spectrometer.

Many experiments at Sandia’s Z Pulsed Power Facility require x-ray backlighting diagnostics to understand experiment performance. Due to limitations in present-day source/detection modalities, most x-ray diagnostics at Z are restricted to photon energies <20 keV, ultimately limiting the density, amount, and atomic number of targets diagnosable in experiments. These limitations force the use of low-Z materials like Beryllium, and they prevent acquisition of important backlighting data for materials/densities that are opaque to soft x-rays and where background emission from the Z load and transmission lines overwhelm diagnostics. In this LDRD project, we have investigated the design and development of a laser wakefield acceleration platform driven by the Z-Petawatt laser – a platform that would enable the generation of a pulsed, collimated beam of high energy x-rays up to 100 keV. Geometrical considerations for implementation on the Z Machine require the use of sacrificial mirrors, which have been tested in offline experiments in the Chama target chamber in building 983. Our results suggest the use of sacrificial mirrors would not necessarily inhibit the laser wakefield x-ray process, particularly with the benefits stemming from planned laser upgrades. These conclusions support the continuation of laser wakefield source research and the development of the necessary infrastructure to deliver the Z-Petawatt laser to the Z center section along the appropriate lines of sight. Ultimately, this new capability will provide unprecedented views through dense states of matter, enabling the use of previously incompatible target materials/designs, and uncovering a new set of observables accessible through diffraction and spectroscopy in the hard x-ray regime. These will amplify the data return on precious Z shots and enhance Sandia’s ability to investigate fundamental physics in support of national security.

We present an overview of the magneto-inertial fusion (MIF) concept MagLIF (Magnetized Liner Inertial Fusion) pursued at Sandia National Laboratories and review some of the most prominent results since the initial experiments in 2013. In MagLIF, a centimeter-scale beryllium tube or "liner" is filled with a fusion fuel, axially pre-magnetized, laser pre-heated, and finally imploded using up to 20 MA from the Z machine. All of these elements are necessary to generate a thermonuclear plasma: laser preheating raises the initial temperature of the fuel, the electrical current implodes the liner and quasi-adiabatically compresses the fuel via the Lorentz force, and the axial magnetic field limits thermal conduction from the hot plasma to the cold liner walls during the implosion. MagLIF is the first MIF concept to demonstrate fusion relevant temperatures, significant fusion production (>10^13 primary DD neutron yield), and magnetic trapping of charged fusion particles. On a 60 MA next-generation pulsed-power machine, two-dimensional simulations suggest that MagLIF has the potential to generate multi-MJ yields with significant self-heating, a long-term goal of the US Stockpile Stewardship Program. At currents exceeding 65 MA, the high gains required for fusion energy could be achievable.

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We report on experimental measurements of how an externally imposed magnetic field affects plasma heating by kJ-class, nanosecond laser pulses. The experiments reported here took place in gas cells analogous to magnetized liner inertial fusion targets. We observed significant changes in laser propagation and energy deposition scale lengths when a 12T external magnetic field was imposed in the gas cell. We find evidence that the axial magnetic field reduces radial electron thermal transport, narrows the width of the heated plasma, and increases the axial plasma length. Reduced thermal conductivity increases radial thermal gradients. This enhances radial hydrodynamic expansion and subsequent thermal self-focusing. Our experiments and supporting 3D simulations in helium demonstrate that magnetization leads to higher thermal gradients, higher peak temperatures, more rapid blast wave development, and beam focusing with an applied field of 12T.

We’re happy to report that the full-aperture upgrade project, started in FY18, is now complete and short-pulse target experiments are underway. The table below lists the present performance level of ZPW. Additional laser improvements are in progress to increase the laser energy and pulse contrast along with implementing a correction for achromatic aberrations to reduce the focused spot size and pulse width.

At the Z Facility at Sandia National Laboratories, the magnetized liner inertial fusion (MagLIF) program aims to study the inertial confinement fusion in deuterium-filled gas cells by implementing a three-step process on the fuel: premagnetization, laser preheat, and Z-pinch compression. In the laser preheat stage, the Z-Beamlet laser focuses through a thin polyimide window to enter the gas cell and heat the fusion fuel. However, it is known that the presence of the few μm thick window reduces the amount of laser energy that enters the gas and causes window material to mix into the fuel. These effects are detrimental to achieving fusion; therefore, a windowless target is desired. The Lasergate concept is designed to accomplish this by "cutting"the window and allowing the interior gas pressure to push the window material out of the beam path just before the heating laser arrives. In this work, we present the proof-of-principle experiments to evaluate a laser-cutting approach to Lasergate and explore the subsequent window and gas dynamics. Further, an experimental comparison of gas preheat with and without Lasergate gives clear indications of an energy deposition advantage using the Lasergate concept, as well as other observed and hypothesized benefits. While Lasergate was conceived with MagLIF in mind, the method is applicable to any laser or diagnostic application requiring direct line of sight to the interior of gas cell targets.

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The high-energy upgrade of the Z-Petawatt (ZPW) laser system involved a shot hiatus starting in October 2018 to allow the installation of full-aperture optics in the chain, including in the main amplifier section as well as in the branches associated with the ZPW compressor and co-injection (the narrowband nanosecond operating mode that is co-bored with Z-Beamlet). Laser shots resumed May 1^st, with most shots since being in the ns mode to reduce complexity (while conditioning optics and calibrating diagnostics) as well as to support experimental requests. To facilitate experimental needs while a final full-sized co-injection optic was prepared, a sub-apertured beam has been used for experimental applications and a full-apertured beam has been used to validate the system. In the latter case, the beam is directed to a large calorimeter placed before branching occurs to the ZPW compressor or co-injection. As of September 2019, full-aperture co-injection shots had ramped up to 960J in 2.3ns, with many cross-calibrations being used to map out a relative humidity dependency in the leaky diagnostic mirror. Several such cross-calibration shots have been done using a chirped pulse seed as well, verifying that the diagnostic calibrations are valid in both broadband and narrow-band modes. Summarizing, since May 1^st of 2019 when shots resumed, 93 full system shots were performed with the ZPW laser. This included 2 co-injection shots with ZBL into Z (in support of MagLIF), 26 Pecos gas cell shots (in support of MagLIF), 11 Conchas gas cell shots (in support of UXI applications development), 6 Jemez shots (in support of backlighter development), and 48 calorimeter shots (in support of validating the system performance). Of these 93 shots, 45 shots were in conjunction with ZBL.

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A multi-frame shadowgraphy diagnostic has been developed and applied to laser preheat experiments relevant to the Magnetized Liner Inertial Fusion (MagLIF) concept. The diagnostic views the plasma created by laser preheat in MagLIF-relevant gas cells immediately after the laser deposits energy as well as the resulting blast wave evolution later in time. The expansion of the blast wave is modeled with 1D radiation-hydrodynamic simulations that relate the boundary of the blast wave at a given time to the energy deposited into the fuel. This technique is applied to four different preheat protocols that have been used in integrated MagLIF experiments to infer the amount of energy deposited by the laser into the fuel. The results of the integrated MagLIF experiments are compared with those of two-dimensional LASNEX simulations. The best performing shots returned neutron yields ∼40-55% of the simulated predictions for three different preheat protocols.

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Dichroic coatings have been developed for high transmission at 527 nm and high reflection at 1054 nm for laser operations in the nanosecond pulse regime. The coatings consist of HfO2 and SiO2 layers deposited with e-beam evaporation, and laser-induced damage thresholds as high as 12.5 J/cm2 were measured at 532 nm with 3.5 ns pulses (22.5 degrees angle of incidence, in S-polarization). However, laser damage measurements at the single wavelength of 532 nm do not adequately characterize the laser damage resistance of these coatings, since they were designed to operate at dual wavelengths simultaneously. This became apparent after one of the coatings damaged prematurely at a lower fluence in the beam train, which inspired further investigations. To gain a more complete understanding of the laser damage resistance, results of a dual-wavelength laser damage test performed at both 532 nm and 1064 nm are presented.

High-intensity lasers interacting with solid foils produce copious numbers of relativistic electrons, which in turn create strong sheath electric fields around the target. The proton beams accelerated in such fields have remarkable properties, enabling ultrafast radiography of plasma phenomena or isochoric heating of dense materials. In view of longer-term multidisciplinary purposes (e.g., spallation neutron sources or cancer therapy), the current challenge is to achieve proton energies well in excess of 100 MeV, which is commonly thought to be possible by raising the on-target laser intensity. Here we present experimental and numerical results demonstrating that magnetostatic fields self-generated on the target surface may pose a fundamental limit to sheath-driven ion acceleration for high enough laser intensities. Those fields can be strong enough (~105 T at laser intensities ~1021 W cm-2) to magnetize the sheath electrons and deflect protons off the accelerating region, hence degrading the maximum energy the latter can acquire.

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A series of Magnetized Liner Inertial Fusion (MagLIF) experiments have been conducted in order to investigate the mix introduced from various target surfaces during the laser preheat stage. The material mixing was measured spectroscopically for a variety of preheat protocols by employing mid-atomic number surface coatings applied to different regions of the MagLIF target. The data show that the material from the top cushion region of the target can be mixed into the fuel during preheat. For some preheat protocols, our experiments show that the laser-entrance-hole (LEH) foil used to contain the fuel can be transported into the fuel a significant fraction of the stagnation length and degrade the target performance. Preheat protocols using pulse shapes of a few-ns duration result in the observable LEH foil mix both with and without phase-plate beam smoothing. In order to reduce this material mixing, a new capability was developed to allow for a low energy (∼20 J) laser pre-pulse to be delivered early in time (-20 ns) before the main laser pulse (∼1.5 kJ). In experiments, this preheat protocol showed no indications of the LEH foil mix. The experimental results are broadly in agreement with pre-shot two-dimensional HYDRA simulations that helped motivate the development of the early pre-pulse capability.

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The Magnetized Liner Inertial Fusion concept (MagLIF) [Slutz et al., Phys. Plasmas 17, 056303 (2010)] is being studied on the Z facility at Sandia National Laboratories. Neutron yields greater than 1012 have been achieved with a drive current in the range of 17-18 MA and pure deuterium fuel [Gomez et al., Phys. Rev. Lett. 113, 155003 (2014)]. We show that 2D simulated yields are about twice the best yields obtained on Z and that a likely cause of this difference is the mix of material into the fuel. Mitigation strategies are presented. Previous numerical studies indicate that much larger yields (10-1000 MJ) should be possible with pulsed power machines producing larger drive currents (45-60 MA) than can be produced by the Z machine [Slutz et al., Phys. Plasmas 23, 022702 (2016)]. To test the accuracy of these 2D simulations, we present modifications to MagLIF experiments using the existing Z facility, for which 2D simulations predict a 100-fold enhancement of MagLIF fusion yields and considerable increases in burn temperatures. Experimental verification of these predictions would increase the credibility of predictions at higher drive currents.

Amplification of the transverse scattered component of stimulated Brillouin scattering (SBS) can contribute to optical damage in the large aperture optics of multi-kJ lasers. Because increased laser bandwidth from optical phase modulation (PM) can suppress SBS, high energy laser amplifiers are injected with PM light. Phase modulation distributes the single-frequency spectrum of a master oscillator laser among individual PM sidebands, so a sufficiently high modulation index β can maintain the fluence for all spectral components below the SBS threshold. To avoid injection of single frequency light in the event of a PM failure, a high-speed PM failsafe system (PMFS) must be employed. Because PM is easily converted to AM, essentially all PM failsafes detect AM, with the one described here employing a novel configuration where optical heterodyne detection converts PM to AM, followed by passive AM power detection. Although the PMFS is currently configured for continuous monitoring, it can also detect PM for pulse durations ≥2 ns and could be modified to accommodate shorter pulses. This PMFS was deployed on the Z-Beamlet Laser (ZBL) at Sandia National Laboratories, as required by an energy upgrade to support programs at Sandia’s Z Facility such as magnetized liner inertial fusion. Depending on the origin of a PM failure, the PMFS responds in as little as 7 ns. In the event of an instantaneous failure during initiation of a laser shot, this response time translates to a 30–50 ns margin of safety by blocking a pulse from leaving ZBL’s regenerative amplifier, which prevents injection of single frequency light into the main amplification chain. In conclusion, the performance of the PMFS, without the need for operator interaction, conforms to the principles of engineered safety.

X-ray diffraction measurements to characterize phase transitions of dynamically compressed high-Z matter at Mbar pressures require both sufficient photon energy and fluence to create data with high fidelity in a single shot. Large-scale laser systems can be used to generate x-ray sources above 10 keV utilizing line radiation of mid-Z elements. However, the laser-to-x-ray energy conversion efficiency at these energies is low, and thermal x-rays or hot electrons result in unwanted background. We employ polycapillary x-ray lenses in powder x-ray diffraction measurements using solid target x-ray emission from either the Z-Beamlet long-pulse or the Z-Petawatt (ZPW) short-pulse laser systems at Sandia National Laboratories. Polycapillary lenses allow for a 100-fold fluence increase compared to a conventional pinhole aperture while simultaneously reducing the background significantly. This enables diffraction measurements up to 16 keV at the few-photon signal level as well as diffraction experiments with ZPW at full intensity.

Existing models for most materials do not describe phase transformations and associated lattice dy- namics (kinetics) under extreme conditions of pressure and temperature. Dynamic x-ray diffraction (DXRD) allows material investigations in situ on an atomic scale due to the correlation between solid-state structures and their associated diffraction patterns. In this LDRD project we have devel- oped a nanosecond laser-compression and picosecond-to-nanosecond x-ray diffraction platform for dynamically-compressed material studies. A new target chamber in the Target Bay in building 983 was commissioned for the ns, kJ Z-Beamlet laser (ZBL) and the 0.1 ns, 250 J Z-Petawatt (ZPW) laser systems, which were used to create 8-16 keV plasma x-ray sources from thin metal foils. The 5 ns, 15 J Chaco laser system was converted to a high-energy laser shock driver to load material samples to GPa stresses. Since laser-to-x-ray energy conversion efficiency above 10 keV is low, we employed polycapillary x-ray lenses for a 100-fold fluence increase compared to a conventional pinhole aperture while simultaneously reducing the background significantly. Polycapillary lenses enabled diffraction measurements up to 16 keV with ZBL as well as diffraction experiments with ZPW. This x-ray diffraction platform supports experiments that are complementary to gas guns and the Z facility due to different strain rates. Ultimately, there is now a foundation to evaluate DXRD techniques and detectors in-house before transferring the technology to Z. This page intentionally left blank.