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Heavy-Ion-Induced Displacement Damage Effects in Magnetic Tunnel Junctions with Perpendicular Anisotropy

IEEE Transactions on Nuclear Science

Xiao, Tianyao X.; Bennett, Christopher H.; Mancoff, Frederick B.; Manuel, Jack E.; Hughart, David R.; Jacobs-Gedrim, Robin B.; Bielejec, Edward S.; Vizkelethy, Gyorgy V.; Sun, Jijun; Aggarwal, Sanjeev; Arghavani, Reza A.; Marinella, Matthew J.

We evaluate the resilience of CoFeB/MgO/CoFeB magnetic tunnel junctions (MTJs) with perpendicular magnetic anisotropy (PMA) to displacement damage induced by heavy-ion irradiation. MTJs were exposed to 3-MeV Ta2+ ions at different levels of ion beam fluence spanning five orders of magnitude. The devices remained insensitive to beam fluences up to $10^{11}$ ions/cm2, beyond which a gradual degradation in the device magnetoresistance, coercive magnetic field, and spin-transfer-torque (STT) switching voltage were observed, ending with a complete loss of magnetoresistance at very high levels of displacement damage (>0.035 displacements per atom). The loss of magnetoresistance is attributed to structural damage at the MgO interfaces, which allows electrons to scatter among the propagating modes within the tunnel barrier and reduces the net spin polarization. Ion-induced damage to the interface also reduces the PMA. This study clarifies the displacement damage thresholds that lead to significant irreversible changes in the characteristics of STT magnetic random access memory (STT-MRAM) and elucidates the physical mechanisms underlying the deterioration in device properties.

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Photocatalytic Material Surfaces for SARS-CoV-2 Virus Inactivation

Negrete, Oscar N.; Bradfute, Steven; Larson, Steven R.; Sinha, Anupama S.; Coombes, Kenneth R.; Goeke, Ronald S.; Keenan, Lisa A.; Duay, Jonathon W.; Van Heukelom, Michael V.; Meserole, Stephen M.; Jacobs-Gedrim, Robin B.

Severe acute respiratory syndrome coronavirus 2 (SARS-COV-2) can be spread through close contact or through fomite mediated transmission. This study details the fabrication and analysis of a photocatalyst surface which can rapidly inactivate SARS-COV-2 to limit spread of the virus by fomite mediated transmission. The surface being developed at Sandia for this purpose is a minimally hazardous Ag-Ti0 2 nanomaterial which is engineered to have high photocatalytic activity. Initial results at Sandia California in a BSL-2 safe surrogate virus- Vesicular Stomatitis Virus (VSV) show a significant difference between the photocatalyst material under exposure to visible light than controls. Additionally, UV-A light (365 nm) was found to eliminate SARS-COV-2 after 9 hours on all tested surfaces with irradiance of 15 mW/cm 2 equivalent to direct circumsolar irradiance.

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COVID-19 LDRD Project Summaries

Treece, Amy T.; Corbin, William C.; Caskey, Susan A.; Krishnakumar, Raga K.; Williams, Kelly P.; Branch, Darren W.; Harmon, Brooke N.; Polsky, Ronen P.; Bauer, Travis L.; Finley, Patrick D.; Jeffers, Robert F.; Safta, Cosmin S.; Makvandi, Monear M.; Laird, Carl D.; Domino, Stefan P.; Ho, Clifford K.; Grillet, Anne M.; Pacheco, Jose L.; Nemer, Martin N.; Rossman, Grant A.; Koplow, Jeffrey P.; Celina, Mathias C.; Jones, Brad H.; Burton, Patrick D.; Haggerty, Ryan P.; Jacobs-Gedrim, Robin B.; Thelen, Paul M.

Sandia National Laboratories currently has 27 COVID-related Laboratory Directed Research & Development (LDRD) projects focused on helping the nation during the pandemic. These LDRD projects cross many disciplines including bioscience, computing & information sciences, engineering science, materials science, nanodevices & microsystems, and radiation effects & high energy density science.

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Comparison of Radiation Effects in Custom-and Commercially-Fabricated Resistive Memory Devices

IEEE Transactions on Nuclear Science

Holt, Joshua S.; Alamgir, Zahiruddin; Beckmann, Karsten; Suguitan, Nadia; Russell, Sierra; Iler, Evan; Bakhru, Hassaram; Bielejec, Edward S.; Jacobs-Gedrim, Robin B.; Hughart, David R.; Marinella, Matthew J.; Yang-Scharlotta, Jean; Cady, Nathaniel C.

The radiation response of TaOx-based RRAM devices fabricated in academic (Set A) and industrial (Set B) settings was compared. Ionization damage from a 60Co gamma source did not cause any changes in device resistance for either device type, up to 45 Mrad(Si). Displacement damage from a heavy ion beam caused the Set B in the high resistance state to decrease in resistance at 1 x 1021 oxygen displacements per cm3; meanwhile, the Set A devices did not exhibit any decrease in resistance due to displacement damage. Both types of devices demonstrated an increase in resistance around 3 x 1022 oxygen displacements per cm3, possibly due to damage at the oxide/metal interfaces. These extremely high levels of damage represent near-total atomic disruption, and if this level of damage were ever reached, other circuit elements would likely fail before the RRAM devices in this study. Generally, both sets of devices were much more resistant to radiation effects than other devices reported in the literature. Displacement damage effects were only observed in the Set A devices once the displacement-induced oxygen vacancies surpassed the intrinsic vacancy concentration in the devices, suggesting that high oxygen vacancy concentration played a role in the devices’ high tolerance to displacement damage.

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Results 1–25 of 63
Results 1–25 of 63