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Importance of cross reaction covariance data for user applications

EPJ Web of Conferences (Online)

Griffin, Patrick J.

The characterization of the uncertainty in radiation damage metrics presents many challenges. This paper examines the current approaches to characterizing radiation damage metrics such as hydrogen and helium gas production, material heating, trapped charge in microelectronics, and lattice displacement damage. Critical uncertainty aspects go beyond just the material cross sections and involve the consideration of energy-dependent cross reaction correlations, the recoil ion energy spectrum, and models used for the partitioning of the recoil ion energy into various forms of energy deposition. This paper starts with a review of terminology and then examines the current approaches in the characterization of uncertainty in radiation damage metrics for several applications. The major deficiencies in the uncertainty of the damage metric characterization are also identified.

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GaAs Neutron Response Functions and Radiation Damage Metrics

Griffin, Patrick J.; Asper, Nicholas; Charlton, William

The radiation effects community needs clear, well-documented, neutron energy-dependent responses that can be used in assessing radiation-induced material damage to GaAs semiconductors and for correlating observed radiation-induced changes in the GaAs electronic properties with computed damage metrics. In support of the objective, this document provides: a) a clearly defined set of relevant neutron response functions for use in dosimetry applications; b) clear mathematical expressions for the defined response functions; and c) updated quantitative values for the energy- dependent response functions that reflect the best current nuclear data and modelling. This document recaps the legacy response functions. It then surveys the latest nuclear data and updates the recommended response function to support current GaAs damage studies. A detailed tabulation for six of the energy-dependent response functions is provided in an Appendix.

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Evaluation of the GaAs Displacement Damage Metric using Updated Nuclear Data

Proceedings of the International Conference on Physics of Reactors, PHYSOR 2022

Asper, Nicholas; Charlton, William; Griffin, Patrick J.

The emerging use of the physics-based athermal recombination-corrected displacement per atom (arc-dpa) model for the displacement damage efficiency has motivated a re-evaluation of the historical empirically-derived GaAs damage response function with the purpose of highlighting needs for future analytical and experimental work. The 1-MeV neutron damage equivalence methodology used in the ASTM E-722 standard for GaAs has been re-evaluated using updated nuclear data. This yielded a higher fidelity representation of the GaAs displacement kerma and, through the use of the refined PKA recoil energy-dependent damage efficiency model, an updated 1-MeV(GaAs) displacement damage function. This re-evaluation included use of the Norgett-Robinson-Torrens (NRT) model for an updated threshold treatment, rather than the sharp-threshold Kinchin-Pease model used in the current ASTM standard. The underlying nuclear data evaluations have been updated to use the ENDF/VIII.0 75As and TENDL-2019 71Ga/69Ga evaluations. The displacement kerma and 1-MeV-equivalent damage responses were calculated using a modified NJOY-2016 code which allowed for refinements in some of the damage models. This paper shows that an updated displacement damage function, based upon the latest nuclear data, is consistent with the experimental data used to develop the current ASTM E-722 GaAs standard. Using a double ratio approach to compare the available experimental data with the calculated response, the average legacy double ratio was found to be 0.97±0.05 and the average updated double ratio was found to be 0.94 ±0.05.

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Evaluation of the GaAs Displacement Damage Metric using Updated Nuclear Data

Proceedings of the International Conference on Physics of Reactors Physor 2022

Asper, Nicholas; Charlton, William; Griffin, Patrick J.

The emerging use of the physics-based athermal recombination-corrected displacement per atom (arc-dpa) model for the displacement damage efficiency has motivated a re-evaluation of the historical empirically-derived GaAs damage response function with the purpose of highlighting needs for future analytical and experimental work. The 1-MeV neutron damage equivalence methodology used in the ASTM E-722 standard for GaAs has been re-evaluated using updated nuclear data. This yielded a higher fidelity representation of the GaAs displacement kerma and, through the use of the refined PKA recoil energy-dependent damage efficiency model, an updated 1-MeV(GaAs) displacement damage function. This re-evaluation included use of the Norgett-Robinson-Torrens (NRT) model for an updated threshold treatment, rather than the sharp-threshold Kinchin-Pease model used in the current ASTM standard. The underlying nuclear data evaluations have been updated to use the ENDF/VIII.0 75As and TENDL-2019 71Ga/69Ga evaluations. The displacement kerma and 1-MeV-equivalent damage responses were calculated using a modified NJOY-2016 code which allowed for refinements in some of the damage models. This paper shows that an updated displacement damage function, based upon the latest nuclear data, is consistent with the experimental data used to develop the current ASTM E-722 GaAs standard. Using a double ratio approach to compare the available experimental data with the calculated response, the average legacy double ratio was found to be 0.97±0.05 and the average updated double ratio was found to be 0.94 ±0.05.

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Response of GaN-Based Semiconductor Devices to Ion and Gamma Irradiation

Aguirre, Brandon A.; King, Joseph; Manuel, Jack; Vizkelethy, Gyorgy; Bielejec, Edward S.; Griffin, Patrick J.

GaN has electronic properties that make it an excellent material for the next generation of power electronics; however, its radiation hardening still needs further understanding before it is used in radiation environments. In this work we explored the response of commercial InGaN LEDs to two different radiation environments: ion and gamma irradiations. For ion irradiations we performed two types of irradiations at the Ion Beam Lab (IBL) at Sandia National Laboratories (SNL): high energy and end of range (EOR) irradiations. For gamma irradiations we fielded devices at the gamma irradiation facility (GIF) at SNL. The response of the LEDs to radiation was investigated by IV, light output and light output vs frequency measurements. We found that dose levels up to 500 krads do not degrade the electrical properties of the devices and that devices exposed to ion irradiations exhibit a linear and non- linear dependence with fluence for two different ranges of fluence levels. We also performed current injection annealing studies to explore the annealing properties of InGaN LEDs.

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DFF Layout Variations in CMOS SOI -Analysis of Hardening by Design Options

IEEE Transactions on Nuclear Science

Black, Jeffrey D.; Black, Dolores A.; Domme, Nicholas A.; Dodd, Paul E.; Griffin, Patrick J.; Nowlin, R.N.; Trippe, James; Salas, Joseph G.; Reed, Robert A.; Weller, Robert A.; Tonigan, Andrew M.; Schrimpf, Ronald D.

Four D flip-flop (DFF) layouts were created from the same schematic in Sandia National Laboratories' CMOS7 silicon-on-insulator (SOI) process. Single-event upset (SEU) modeling and testing showed an improved response with the use of shallow (not fully bottomed) N-type metal-oxide-semiconductor field-effect transistors (NMOSFETs), extending the size of the drain implant and increasing the critical charge of the transmission gates in the circuit design and layout. This research also shows the importance of correctly modeling nodal capacitance, which is a major factor determining SEU critical charge. Accurate SEU models enable the understanding of the SEU vulnerabilities and how to make the design more robust.

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IRDFF-II: A New Neutron Metrology Library

Nuclear Data Sheets

Griffin, Patrick J.; Trkov, A.; Simakov, S.P.; Greenwood, L.R.; Zolotarev, K.I.; Capote, R.; Destouches, C.; Kahler, A.C.; Konno, C.; Kostal, M.; Aldama, D.L.; Chechev, V.; Majerle, M.; Malambu, E.; Ohta, M.; Pronyaev, V.G.; Yashima, H.; White, M.; Wagemans, J.; Vavtar, I.; Simeckova, E.; Radulovic, V.; Sato, S.

High quality nuclear data is the most fundamental underpinning for all neutron metrology applications. This paper describes the release of version II of the International Reactor Dosimetry and Fusion File (IRDFF-II) that contains a consistent set of nuclear data for fission and fusion neutron metrology applications up to 60 MeV neutron energy. The library is intended to support: a) applications in research reactors; b) safety and regulatory applications in the nuclear power generation in commercial fission reactors; and c) material damage studies in support of the research and development of advanced fusion concepts. The paper describes the contents of the library, documents the thorough verification process used in its preparation, and provides an extensive set of validation data gathered from a wide range of neutron benchmark fields. The new IRDFF-II library includes 119 metrology reactions, four cover material reactions to support self-shielding corrections, five metrology metrics used by the dosimetry community, and cumulative fission products yields for seven fission products in three different neutron energy regions. In support of characterizing the measurement of the residual nuclei from the dosimetry reactions and the fission product decay modes, the present document lists the recommended decay data, particle emission energies and probabilities for 68 activation products. It also includes neutron spectral characterization data for 29 neutron benchmark fields for the validation of the library contents. Additional six reference fields were assessed (four from plutonium critical assemblies, two measured fields for thermal-neutron induced fission on 233U and 239Pu targets) but not used for validation due to systematic discrepancies in C/E reaction rate values or lack of reaction-rate experimental data. Another ten analytical functions are included that can be useful for calculating average cross sections, average energy, thermal spectrum average cross sections and resonance integrals. The IRDFF-II library and comprehensive documentation is available online at www-nds.iaea.org/IRDFF/. Evaluated cross sections can be compared with experimental data and other evaluations at www-nds.iaea.org/exfor/endf.htm. The new library is expected to become the international reference in neutron metrology for multiple applications.

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RML Dosimetry Conversions for SNL Reference Benchmark Neutron Fields

Griffin, Patrick J.; Parma, Edward J.; Vega, Richard M.; Vehar, David W.

Neutron dosimetry monitors should be used during all irradiations in the Annular Core Research Reactor. This report provides the recommended conversion factors that should be used to translate the monitor dosimeter read-outs into the damage metrics that are typically used by experimenters to assess the results of their experiment. These conversion factors are based upon the use of the latest least-squares adjusted neutron spectrum determination to describe the Sandia National Laboratories reference neutron fields and the latest International Atomic Energy Agency recommended dosimetry cross sections to capture the response of the dosimeter. The resulting conversion factors are built into the dosimetry results routinely provided by the Radiation Metrology Laboratory.

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Uncertainty Characterization of Silicon Damage Metrics

IEEE Transactions on Nuclear Science

Griffin, Patrick J.

A general formulation of silicon damage metrics and associated energy-dependent response functions relevant to the radiation effects community is provided. Using this formulation, a rigorous quantitative treatment of the energy-dependent uncertainty contributors is performed. This resulted in the generation of a covariance matrix for the displacement kerma, the Norgett-Robinson-Torrens-based damage energy, and the 1-MeV(Si)-equivalent damage function. When a careful methodology is used to apply a reference 1-MeV damage value, the systematic uncertainty in the fast fission region is seen to be removed, and the uncertainty for integral metrics in broad-based fission-based neutron fields is demonstrated to be significantly reduced.

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Uncertainty Characterization of Silicon Damage Metrics

IEEE Transactions on Nuclear Science

Griffin, Patrick J.

Here, a general formulation of silicon damage metrics and associated energy-dependent response functions relevant to the radiation effects community is provided. Using this formulation, a rigorous quantitative treatment of the energy-dependent uncertainty contributors is performed. This resulted in the generation of a covariance matrix for the displacement kerma, the NRT-based damage energy, and the 1-MeV(Si) equivalent damage function. Lastly, when a careful methodology is used to apply a reference 1-MeV damage value, the systematic uncertainty in the fast fission region is seen to be removed and the uncertainty for integral metrics in broad-based fission-based neutron fields is demonstrated to be significantly reduced.

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Importance of treating correlations in the uncertainty quantification of radiation damage metrics

20th Topical Meeting of the Radiation Protection and Shielding Division, RPSD 2018

Griffin, Patrick J.; Koning, Arjan; Rochman, Dimitri

The radiation effects community embraces the importance of quantifying uncertainty in model predictions and the importance of propagating this uncertainty into the integral metrics used to validate models, but they are not always aware of the importance of addressing the energy- and reaction-dependent correlations in the underlying uncertainty contributors. This paper presents a rigorous high-fidelity Total Monte Carlo approach that addresses the correlation in the underlying uncertainty components and quantifies the role of both energy and reaction-dependent correlations in a sample application that addresses the damage metrics relevant to silicon semiconductors.

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Correlation of a Bipolar-Transistor-Based Neutron Displacement Damage Sensor Methodology with Proton Irradiations

IEEE Transactions on Nuclear Science

Tonigan, Andrew M.; Arutt, Charles N.; Parma, Edward J.; Griffin, Patrick J.; Schrimpf, Ronald D.

A bipolar-transistor-based sensor technique has been used to compare silicon displacement damage from known and unknown neutron energy spectra generated in nuclear reactor and high-energy-density physics environments. The technique has been shown to yield 1-MeV(Si) equivalent neutron fluence measurements comparable to traditional neutron activation dosimetry. This paper significantly extends previous results by evaluating three types of bipolar devices utilized as displacement damage sensors at a nuclear research reactor and at a Pelletron particle accelerator. Ionizing dose effects are compensated for via comparisons with 10-keV X-ray and/or cobalt-60 gamma ray irradiations. Nonionizing energy loss calculations adequately approximate the correlations between particle and device responses and provide evidence for the use of one particle type to screen the sensitivity of the other.

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Characterization of the energy-dependent uncertainty and correlation in silicon neutron displacement damage metrics

EPJ Web of Conferences

Griffin, Patrick J.; Rochman, Dimitri; Koning, Arjan

A rigorous treatment of the uncertainty in the underlying nuclear data on silicon displacement damage metrics is presented. The uncertainty in the cross sections and recoil atom spectra are propagated into the energy-dependent uncertainty contribution in the silicon displacement kerma and damage energy using a Total Monte Carlo treatment. An energy-dependent covariance matrix is used to characterize the resulting uncertainty. A strong correlation between different reaction channels is observed in the high energy neutron contributions to the displacement damage metrics which supports the necessity of using a Monte Carlo based method to address the nonlinear nature of the uncertainty propagation.

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Radiation Characterization Summary: ACRR-FRECII Cavity Free-Field Environment at the Core Centerline (ACRR-FRECII-FF-cl)

Parma, Edward J.; Naranjo, Gerald E.; Lippert, Lance L.; Clovis, Ralph D.; Martin, Lonnie E.; Kaiser, Krista I.; Emmer, Joshua; Greenberg, Joseph; Klein, James O.; Quirk, Thomas J.; Vehar, David W.; Griffin, Patrick J.

This document presents the facility - recommended characterization of the neutron, prompt gamma - ray, and delayed gamma - ray radiation fields in the Annular Core Research Reactor ( ACRR ) Fueled - Ring External Cavity II (FREC - II) for the free - field environment at the core centerline. The designation for this environment is ACRR - FRECII - FF - cl. The neutron, prompt gamma - ray, and delayed gamma - ray energy spectra, uncertainties, and covariance matrices are presented as well as radial and axial neutron and gamma - ray fluence profiles within the experiment area of the cavity. Recommended constants are given to facilitate the conversion of various dosimetry readings into radiation metrics desired by experimenters. Representative pulse operations are presented with conversion examples.

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Influence of the Damage Partition Function on the Uncertainty of the Silicon Displacement Damage Metric

IEEE Transactions on Nuclear Science

Griffin, Patrick J.; Cooper, Philip J.

The effect of uncertainty in the energy partition function on the silicon displacement damage metric is presented. Through the use of a Total Monte Carlo approach, the effect of uncertainty in the underlying electronic and nuclear ion interaction potentials, which are used to define the damage partition function, is propagated into an uncertainty in the silicon damage metric. This uncertainty is expressed as an energy-dependent covariance matrix which permits this uncertainty component to be combined with other uncertainty components, e.g. uncertainty due to the knowledge of the nuclear interaction data or to the treatment of the damage in the threshold displacement region. This approach provides a rigorous treatment of uncertainty due to the damage metric which can then be propagated in uncertainty estimates for various applications, e.g. when examining damage equivalence between different neutron sources. A strong energy-dependent correlation is found in this uncertainty component.

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Detailed Description of the Derivation of the Silicon Damage Response Function

Griffin, Patrick J.

This report provides a set of consistent definitions for radiation damage metrics relevant to the modeling of displacement damage in materials. The limitations/approximations built into the various metrics are discussed, as are the intended applications that gave rise to community use of the damage metrics. Numerical tabulations are provided, based on the latest nuclear data, for recommended values of the neutron displacement kerma factor and various NRT-based damage energy metrics in silicon.

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Validation of IRDFF in 252Cf Standard and IRDF-2002 Reference Neutron Fields

EPJ Web of Conferences

Griffin, Patrick J.; Simakov, Stanislav; Capote, Roberto; Greenwood, Lawrence; Kahler, Albert; Trkov, Andrej; Zolotarev, Konstantin; Pronyaev, Vladimir

The results of validation of the latest release of International Reactor Dosimetry and Fusion File, IRDFF-1.03, in the standard 252Cf(s.f.) and reference 235U(nth,f) neutron benchmark fields are presented. The spectrum-averaged cross sections were shown to confirm IRDFF-1.03 in the 252Cf standard spontaneous fission spectrum; that was not the case for the current recommended spectra for 235U(nth,f). IRDFF was also validated in the spectra of the research reactor facilities ISNF, Sigma-Sigma and YAYOI, which are available in the IRDF-2002 collection. The ISNF facility was re-simulated to remove unphysical oscillations in the spectrum. IRDFF-1.03 was shown to reproduce reasonably well the spectrum-averaged data measured in these fields except for the case of YAYOI.

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Advanced UQ approaches to the validation of the IRDFF library

Physics of Reactors 2016, PHYSOR 2016: Unifying Theory and Experiments in the 21st Century

Griffin, Patrick J.; Parma, Edward J.; Vehar, David W.

The IRDFF cross section library provides the highest fidelity cross section characterization and is the recommended data library to be used for dosimetry in support of reactor pressure vessel surveillance programs. In order to support this critical application, quantified validation evidence is required for the cross section library. Results are reported here on the use of various advanced approaches to uncertainty quantification using metrics relevant to spectrum characterization applications. The use of a quantified least squares approach, combining a consistent treatment of uncertainty from the spectral characterizations, the dosimetry cross sections, and measured activation products, is identified as one of the most sensitive metrics by which to report validation evidence. Using this metric the status of the validation of the IRDFF library was investigated. This analysis began with a consideration of the best characterized 252Cf spontaneous fission standard neutron benchmark field. Good validation evidence is found for 39 of the 79 IRDFF reactions. The 235U thermal fission reference neutron field was then investigated, and found to yield good validation evidence for an additional 10 of the IRDFF reactions. Extending the analysis further to include four different reactor-based reference neutron benchmark fields, ranging from fast burst reactors to well-moderated pool-type reactors, yielded good validation evidence for an additional 6 IRDFF reactions. In total, evidence is reported here for 55 of the 79 reactions in the IRDFF library.

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Radiation Characterization Summary: ACRR Central Cavity Free-Field Environment with the 32-Inch Pedestal at the Core Centerline (ACRR-FF-CC-32-cl)

Vega, Richard M.; Parma, Edward J.; Naranjo, Gerald E.; Lippert, Lance L.; Vehar, David W.; Griffin, Patrick J.

This document presents the facility-recommended characterization of the neutron, prompt gamma-ray, and delayed gamma-ray radiation fields in the Annular Core Research Reactor (ACRR) for the central cavity free-field environment with the 32-inch pedestal at the core centerline. The designation for this environment is ACRR-FF-CC-32-cl. The neutron, prompt gamma-ray, and delayed gamma-ray energy spectra, uncertainties, and covariance matrices are presented as well as radial and axial neutron and gamma-ray fluence profiles within the experiment area of the cavity. Recommended constants are given to facilitate the conversion of various dosimetry readings into radiation metrics desired by experimenters. Representative pulse operations are presented with conversion examples.

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Neutron Reference Benchmark Field Specifications: ACRR Polyethylene-Lead-Graphite (PLG) Bucket Environment (ACRR-PLG-CC-32-CL)

Vega, Richard M.; Parma, Edward J.; Griffin, Patrick J.; Vehar, David W.

This report was put together to support the International Atomic Energy Agency (IAEA) REAL- 2016 activity to validate the dosimetry community’s ability to use a consistent set of activation data and to derive consistent spectral characterizations. The report captures details of integral measurements taken in the Annular Core Research Reactor (ACRR) central cavity with the Polyethylene-Lead-Graphite (PLG) bucket, reference neutron benchmark field. The field is described and an “a priori” calculated neutron spectrum is reported, based on MCNP6 calculations, and a subject matter expert (SME) based covariance matrix is given for this “a priori” spectrum. The results of 37 integral dosimetry measurements in the neutron field are reported.

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Neutron Reference Benchmark Field Specification: ACRR 44 Inch Lead-Boron (LB44) Bucket Environment (ACRR-LB44-CC-32-CL)

Vega, Richard M.; Parma, Edward J.; Griffin, Patrick J.; Vehar, David W.

This report was put together to support the International Atomic Energy Agency (IAEA) REAL- 2016 activity to validate the dosimetry community’s ability to use a consistent set of activation data and to derive consistent spectral characterizations. The report captures details of integral measurements taken in the Annular Core Research Reactor (ACRR) central cavity with the 44 inch Lead-Boron (LB44) bucket, reference neutron benchmark field. The field is described and an “a priori” calculated neutron spectrum is reported, based on MCNP6 calculations, and a subject matter expert (SME) based covariance matrix is given for this “a priori” spectrum. The results of 31 integral dosimetry measurements in the neutron field are reported.

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Neutron Reference Benchmark Field Specification: ACRR Free-Field Environment (ACRR-FF-CC-32-CL)

Vega, Richard M.; Parma, Edward J.; Griffin, Patrick J.; Vehar, David W.

This report was put together to support the International Atomic Energy Agency (IAEA) REAL- 2016 activity to validate the dosimetry community’s ability to use a consistent set of activation data and to derive consistent spectral characterizations. The report captures details of integral measurements taken in the Annular Core Research Reactor (ACRR) central cavity free-field reference neutron benchmark field. The field is described and an “a priori” calculated neutron spectrum is reported, based on MCNP6 calculations, and a subject matter expert (SME) based covariance matrix is given for this “a priori” spectrum. The results of 31 integral dosimetry measurements in the neutron field are reported.

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Radiation Characterization Summary: ACRR Polyethylene-Lead-Graphite (PLG) Bucket Located in the Central Cavity on the 32-Inch Pedestal at the Core Centerline (ACRR-PLG-CC-32-cl)

Parma, Edward J.; Vehar, David W.; Lippert, Lance L.; Griffin, Patrick J.; Naranjo, Gerald E.; Luker, Spencer M.

This document presents the facility-recommended characterization of the neutron, prompt gamma-ray, and delayed gamma-ray radiation fields in the Annular Core Research Reactor (ACRR) for the polyethylene-lead-graphite (PLG) bucket in the central cavity on the 32-inch pedestal at the core centerline. The designation for this environment is ACRR-PLG-CC-32-cl. The neutron, prompt gamma-ray, and delayed gamma-ray energy spectra, uncertainties, and covariance matrices are presented as well as radial and axial neutron and gamma-ray fluence profiles within the experiment area of the bucket. Recommended constants are given to facilitate the conversion of various dosimetry readings into radiation metrics desired by experimenters. Representative pulse operations are presented with conversion examples. Acknowledgements The authors wish to thank the Annular Core Research Reactor staff and the Radiation Metrology Laboratory staff for their support of this work. Also thanks to David Ames for his assistance in running MCNP on the Sandia parallel machines.

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Covariance propagation in spectral indices

Nuclear Data Sheets

Griffin, Patrick J.

In this study, the dosimetry community has a history of using spectral indices to support neutron spectrum characterization and cross section validation efforts. An important aspect to this type of analysis is the proper consideration of the contribution of the spectrum uncertainty to the total uncertainty in calculated spectral indices (SIs). This study identifies deficiencies in the traditional treatment of the SI uncertainty, provides simple bounds to the spectral component in the SI uncertainty estimates, verifies that these estimates are reflected in actual applications, details a methodology that rigorously captures the spectral contribution to the uncertainty in the SI, and provides quantified examples that demonstrate the importance of the proper treatment the spectral contribution to the uncertainty in the SI.

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Relationship between Metrics Used to Represent Displacement Damage in Materials

Griffin, Patrick J.

This report provides a set of consistent definitions for metrics relevant to the modeling of displacement damage in materials. The limitations/approximations built into the various metrics are discussed as is the intended application that gave rise to community use of the metric. Recommended sources for numerical tabulations of the neutron displacement kerma and the charged particle non-ionizing energy loss in some important semiconductor materials are also provided.

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Radiation characterization summary :

Parma, Edward J.; Lippert, Lance L.; Griffin, Patrick J.; Naranjo, Gerald E.; Luker, Spencer M.

This document presents the facility-recommended characterization of the neutron, prompt gamma-ray, and delayed gamma-ray radiation fields in the Annular Core Research Reactor (ACRR) for the 44-inch-long lead-boron bucket in the central cavity on the 32-inch pedestal at the core centerline. The designation for this environment is ACRR-LB44-CC-32-cl. The neutron, prompt gamma-ray, and delayed gamma-ray energy spectra are presented as well as radial and axial neutron and gamma-ray flux profiles within the experiment area of the bucket. Recommended constants are given to facilitate the conversion of various dosimetry readings into radiation metrics desired by experimenters. Representative pulse and steady-state operations are presented with conversion examples.

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EPR/PTFE dosimetry for test reactor environments

Journal of ASTM International

Vehar, David W.; Griffin, Patrick J.; Quirk, Thomas J.

In 1992 the Radiation Metrology Laboratory (RML) at Sandia National Laboratories implemented EPR/Alanine capabilities for use in routine and calibration activities at its Co-60 and pulsed-power facilities. At that time it also investigated the usefulness of the system for measurement of absorbed dose in the mixed neutron/photon environments of reactors such as the Sandia Pulsed Reactor and the Annular Core Research Reactor used for hardness testing of electronics. The RML concluded that the neutron response of alanine was a sufficiently high fraction of the overall dosimeter response that the resulting uncertainties in the photon dose would be unacceptably large for silicon-device testing. However, it also suggested that non-hydrogenous materials such as polytetrafluoroethylene (PTFE) would exhibit smaller neutron response and might be useful in mixed environments. Preliminary research with PTFE in photon environments indicated considerable promise, but further development was not pursued at that time. Because of renewed interest in absorbed dose measurements that could better define the individual contributions of photon and neutron components to the overall dose delivered to a test object, the RML has re-initiated the development of an EPR/PTFE dosimetry system. This paper presents a summary of the research, a description of the EPR/PTFE dosimetry system, and recommendations for preparation and fielding of the dosimetry in photon and mixed neutron/photon environments. Copyright © 2012 by ASTM International.

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Path forward for dosimetry cross sections

ASTM Special Technical Publication

Griffin, Patrick J.; Peters, C.D.

In the 1980's the dosimetry community embraced the need for a high fidelity quantification of uncertainty in nuclear data used for dosimetry applications. This led to the adoption of energy-dependent covariance matrices as the accepted manner of quantifying the uncertainty data. The trend for the dosimetry community to require high fidelity treatment of uncertainty estimates has continued to the current time where requirements on nuclear data are codified in standards such as ASTM E 1018. This paper surveys the current state of the dosimetry cross sections and investigates the quality of the current dosimetry cross section evaluations by examining calculated-to-experimental ratios in neutron benchmark fields. In recent years more nuclear-related technical areas are placing an emphasis on uncertainty quantification. With the availability of model-based cross sections and covariance matrices produced by nuclear data codes, some nuclear-related communities are considering the role these covariance matrices should play. While funding within the dosimetry community for cross section evaluations has been very meager, other areas, such as the solar-related astrophysics community and the US Nuclear Criticality Safety Program, have been supporting research in the area of neutron cross sections. The Cross Section Evaluation Working Group (CSEWG) is responsible for the creation and maintenance of the ENDF/B library which has been the mainstay for the reactor dosimetry community. Given the new trends in cross section evaluations, this paper explores the path forward for the US nuclear reactor dosimetry community and its use of the ENDF/B cross-sections. The major concern is maintenance of the sufficiency and accuracy of the uncertainty estimate when used for dosimetry applications. The two major areas of deficiency in the proposed ENDF/B approach are: 1) the use of unrelated covariance matrices in ENDF/B evaluations and 2) the lack of "due consideration" of experimental data in the evaluation. Copyright © 2012 by ASTM International.

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Ground water and snow sensor based on directional detection of cosmogenic neutrons

Griffin, Patrick J.; Marleau, P.

A fast neutron detector is being developed to measure the cosmic ray neutron flux in order to measure soil moisture. Soil that is saturated with water has an enhanced ability to moderate fast neutrons, removing them from the backscatter spectrum. The detector is a two-element, liquid scintillator detector. The choice of liquid scintillator allows rejection of gamma background contamination from the desired neutron signal. This enhances the ability to reconstruct the energy and direction of a coincident neutron event. The ability to image on an event-by-event basis allows the detector to selectively scan the neutron flux as a function of distance from the detector. Calibrations, simulations, and optimization have been completed to understand the detector response to neutron sources at variable distances and directions. This has been applied to laboratory background measurements in preparation for outdoor field tests.

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Development of a silicon calorimeter for dosimetry applications in a water-moderated reactor

ASTM Special Technical Publication

Luker, Spencer M.; Griffin, Patrick J.; Depriest, Kendall R.; King, Donald B.; Naranjo, Gerald E.; Suo-Anttila, Ahti J.; Kellner, Ned

High fidelity active dosimetry in the mixed neutron/gamma field of a research reactor is a very complex issue. For passive dosimetry applications, the use of activation foils addresses the neutron environment while the use of low neutron response CaF2:Mn thermoluminescent dosimeters (TLDs) addresses the gamma environment. While radiation-hardened diamond photoconducting detectors (PCD) have been developed that provide a very precise fast response (picosecond) dosimeter and can provide a time-dependent profile for the radiation environment, the mixed field response of the PCD is still uncertain and this interferes with the calibration of the PCD response. In order to address the research reactor experimenter's need for a dosimeter that reports silicon dose and dose rate at a test location during a pulsed reactor operation, a silicon calorimeter has been developed. This dosimeter can be used by itself to provide a dose in rad(Si) up to a point in a reactor pulsed operation, or, in conjunction with the diamond PCD, to provide a dose rate. This paper reports on the development, testing, and validation of this silicon calorimeter for applications in water-moderated research reactors. Copyright © 2006 by ASTM International.

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Neutron Contribution to CaF2:Mn Thermoluminescent Dosimeter Response in Mixed (n/γ) Field Environments

IEEE Transactions on Nuclear Science

Depriest, Kendall R.; Griffin, Patrick J.

Thermoluminescent dosimeters (TLDs), particularly CaF2:Mn, are often used as photon dosimeters in mixed (n/γ) field environments. In these mixed field environments, it is desirable to separate the photon response of a dosimeter from the neutron response. For passive dosimeters that measure an integral response, such as TLDs, the separation of the two components must be performed by postexperiment analysis because the TLD reading system cannot distinguish between photon- and neutron-produced response. Using a model of an aluminum-equilibrated TLD-400 (CaF2:Mn) chip, a systematic effort has been made to analytically determine the various components that contribute to the neutron response of a TLD reading. The calculations were performed for five measured reactor neutron spectra and one theoretical thermal neutron spectrum. The five measured reactor spectra all have experimental values for aluminum-equilibrated TLD-400 chips. Calculations were used to determine the percentage of the total TLD response produced by neutron interactions in the TLD and aluminum equilibrator. These calculations will aid the Sandia National Laboratories-Radiation Metrology Laboratory (SNL-RML) in the interpretation of the uncertainty for TLD dosimetry measurements in the mixed field environments produced by SNL reactor facilities.

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Criteria for the Selection of Dosimetry Cross Sections

IEEE Transactions on Nuclear Science

Griffin, Patrick J.

This paper defines a process for selecting dosimetry-quality cross sections. The recommended cross-section evaluation depends on screening high-quality evaluations with quantified uncertainties, down-selecting based on comparison to experiments in standard neutron fields, and consistency checking in reference neutron fields. This procedure is illustrated for the 23Na(n, γ)24 Na reaction.

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ASTM standards for reactor dosimetry and pressure vessel surveillance

ASTM Special Technical Publication

Griffin, Patrick J.

The ASTM standards provide guidance and instruction on how to field and interpret reactor dosimetry. They provide a roadmap towards understanding the current "state-of-the-art" in reactor dosimetry, as reflected by the technical community. The consensus basis to the ASTM standards assures the user of an unbiased presentation of technical procedures and interpretations of the measurements. Some insight into the types of standards and the way in which they are organized can assist one in using them in an expeditious manner. Two examples are presented to help orient new users to the breadth and interrelationship between the ASTM nuclear metrology standards. One example involves the testing of a new "widget" to verify the radiation hardness. The second example involves quantifying the radiation damage at a pressure vessel critical weld location through surveillance dosimetry and calculation.

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Review of the Palisades pressure vessel accumulated fluence estimate and of the least squares methodology employed

Griffin, Patrick J.

This report provides a review of the Palisades submittal to the Nuclear Regulatory Commission requesting endorsement of their accumulated neutron fluence estimates based on a least squares adjustment methodology. This review highlights some minor issues in the applied methodology and provides some recommendations for future work. The overall conclusion is that the Palisades fluence estimation methodology provides a reasonable approach to a {open_quotes}best estimate{close_quotes} of the accumulated pressure vessel neutron fluence and is consistent with the state-of-the-art analysis as detailed in community consensus ASTM standards.

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Application of reactors for testing neutron-induced upsets in commercial SRAMs

Griffin, Patrick J.

Reactor neutron environments can be used to test/screen the sensitivity of unhardened commercial SRAMs to low-LET neutron-induced upset. Tests indicate both thermal/epithermal (< 1 keV) and fast neutrons can cause upsets in unhardened parts. Measured upset rates in reactor environments can be used to model the upset rate for arbitrary neutron spectra.

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Uncertainty of silicon 1-MeV damage function

Griffin, Patrick J.

The electronics radiation hardness-testing community uses the ASTM E722-93 Standard Practice to define the energy dependence of the nonionizing neutron damage to silicon semiconductors. This neutron displacement damage response function is defined to be equal to the silicon displacement kerma as calculated from the ORNL Si cross-section evaluation. Experimental work has shown that observed damage ratios at various test facilities agree with the defined response function to within 5%. Here, a covariance matrix for the silicon 1-MeV neutron displacement damage function is developed. This uncertainty data will support the electronic radiation hardness-testing community and will permit silicon displacement damage sensors to be used in least squares spectrum adjustment codes.

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Comparison of calculated and experimental dosimetry activities for benchmark neutron fields

Griffin, Patrick J.

New dosimetry cross-section evaluations have been made available to the reactor community. Most dosimetry-quality evaluations include a section (File 33) that defines the uncertainty and covariance matrix for the dosimetry reaction cross section. This paper compares the latest computed cross-section activities for benchmark neutron fields with experimental data. Uncertainty data is usually reported with experimental measurements. This work also presents uncertainty data for the calculated activities. The calculated uncertainty values include a full uncertainty propagation using the cross-section evaluation, energy-dependent covariance data as well as the uncertainty attributed to the knowledge of the neutron spectrum.

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Factors affecting use of fission foils as dosimetry sensors

Griffin, Patrick J.

Fission foils are commonly used as dosimetry sensors. They play a very important role in neutron spectrum determinations. This paper provides a combination of experimental measurements and calculations to quantify the importance and synergy of several factors that affect the fission response of a dosimeter. Only when these effects are properly treated can fission dosimeters be used with sufficient fidelity.

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An ``exact`` treatment of self-shielding and covers in neutron spectra determinations

Griffin, Patrick J.

Most neutron spectrum determination methodologies ignore self-shielding effects in dosimetry foils and treat covers with an exponential attenuation model. This work provides a quantitative analysis of the approximations in this approach. It also provides a methodology for improving the fidelity of the treatment of the dosimetry sensor response to a level consistent with the user`s spectrum characterization approach. A library of correction functions for the energy-dependent sensor response has been compiled that addresses dosimetry foils/configurations in use at the Sandia National Laboratories Radiation Metrology Laboratory.

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Effect of New Cross Section Evaluations on Neutron Spectrum Determination

IEEE Transactions on Nuclear Science

Griffin, Patrick J.

Several new neutron cross section libraries, such as ENDF/ B-VI and IRDF-90, have recently been made available to the dosimetry community. Recommendations are made for the source selection of reaction cross sections that vary significantly among the libraries. In general, integral parameters from spectra obtained from unfold/adjustment codes using the new cross sections will not significantly change. A 61-reaction compendium of dosimetry cross sections drawn from existing evaluations has been compiled for use at the Sandia National Laboratories Radiation Metrology Laboratory. This dosimetry library (SNLRML) is recommended for use in spectrum determination with unfold/ adjustment methods. © 1992 IEEE

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Neutron damage equivalence in GaAs

IEEE Transactions on Nuclear Science

Griffin, Patrick J.

A 1-MeV neutron damage equivalence methodology and damage function have been developed for GaAs based on a recoil-energy dependent damage efficiency and the displacement kerma. This method, developed using life-time degradation in GaAs LEDs in a variety of neutron spectra, is also shown to be applicable to carrier removal. A validated methodology, such as this, is required to ensure and evaluate simulation fidelity in the neutron testing of GaAs semiconductors.

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Effect of ENDF/B-VI cross sections on neutron dosimetry

Griffin, Patrick J.

ENDF/B-VI cross sections were released to the testing community in January 1990. Work at Sandia National Laboratories, with pre-released versions of the new cross sections indicates that changes in the neutron-induced charged-particle reactions will significantly affect 14-MeV neutron dosimetry. Reactions that are important for fission reactor dosimetry were examined and most did not change significantly. 12 refs., 3 figs., 3 tabs.

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94 Results
94 Results