Publications

Heavy particle radiation can produce upsets in digital circuits as well as trigger burn out or breakdown in power MOSFETs and MNOS nonvolatile memories. Latch-up may also be stimulated by heavy ions. This report covers work done on the effects of heavy particle radiation on PN junctions, CMOS inverters, CMOS latch, MOSFET and non-volatile memories. 15 refs., 3 figs.

In this study, we explored several ways of extending SP-100 reactor technology to higher power levels. One approach was to use the reference SP-100 pin design and increase the fuel pin length and the number of fuel pins as needed to provide higher capability. The impact on scaling of a modified and advanced SP-100 reactor technology was also explored. Finally, the effect of using alternative power conversion subsystems, with SP-100 reactor technology was investigated. One of the principal concerns for any space-based system is mass; consequently, this study focused on estimating reactor, shield, and total system mass. The RSMASS code (Marshall 1986) was used to estimate reactor and shield mass. Simple algorithms developed at NASA Lewis Research Center were used to estimate the balance of system mass. Power ranges from 100 kWe to 10 MWe were explored assuming both one year and seven years of operation. Thermoelectric, Stirling, Rankine, and Brayton power conversion systems were investigated. The impact on safety, reliability, and other system attributes, caused by extending the technology to higher power levels, was also investigated. 6 refs., 4 figs., 3 tabs.

Outlier samples can have very detrimental effects on the performances of multivariate calibration methods, as these methods are generally not very robust. Often, the software implementations of these methods do not check for outliers. If outliers are not detected, invalid predictions may result. This paper illustrates some simple exploratory procedures for detecting outliers with examples from near-infrared and mid-infrared spectroscopy using partial least-squares regression as the calibration method. 8 refs., 9 figs., 1 tab.

The experiments described here indicate when one of Nature's best fractals -- the Brownian trail -- becomes nonfractal. In most ambient fluids, the trail of a Brownian particle is self-similar over many decades of length. For example, the trail of a submicron particle suspended in an ordinary liquid, recorded at equal time intervals, exhibits apparently discontinuous changes in velocity from macroscopic lengths down to molecular lengths: the trail is a random walk with no velocity memory'' from one step to the next. In ideal Brownian motion, the kinks in the trail persist to infinitesimal time intervals, i.e., it is a curve without tangents. Even in real Brownian motion in a liquid, the time interval must be shortened to {approximately}10{sup {minus}8}s before the velocity appears continuous. In sufficiently rarefied environments, this time resolution at which a Brownian trail is rectified from a curve without tangents to a smoothly varying trajectory is greatly lengthened, making it possible to study the kinetic regime by dynamic light scattering. Our recent experiments with particles in a plasma have demonstrated this capability. In this regime, the particle velocity persists over a finite step length'' allowing an analogy to an ideal gas with Maxwell-Boltzmann velocities; the particle mass could be obtained from equipartition. The crossover from ballistic flight to hydrodynamic diffusion was also seen. 8 refs., 1 fig.

The MELCOR computer code, which has been developed at Sandia National Laboratories for the US Nuclear Regulatory Commission as a tool for calculating realistic estimates of severe accident consequences and source terms, has been used to analyze a series of containment issues for station blackout sequences for the Grand Gulf Nuclear Power Plant. The results indicate that there is a limited time interval in which the drywell atmosphere would be flammable, and that this would only occur if the vacuum breaker were to stick open within a narrow time window. If burning does occur during this time, it appears quite likely that it would not pose a threat to the drywell wall. The main conclusion from this study is that the drywell atmosphere is not very likely to be flammable for a station blackout sequence. 1 ref. (S.J.)

The influence of postweld heat treatment (PWHT) on the structure, mechanical properties and fracture characteristics of pulsed, Nd: YAG laser welds in a Ti-14.8 wt % Al-21.3 wt % Nb titanium aluminide has been investigated. Significant microstructure variations within the fusion zone (FZ) of all heat-treated welds were attributed primarily to the influence of local compositional fluctuations on decomposition of the metastable-{beta} microstructure present in the as-welded FZ. An increase in PWHT temperature promoted a decrease in the maximum FZ hardness and an increase in the longitudinal-weld bend ductility. Correspondingly, the proportion of ductile tearing to cleavage fracture within the FZ increased with an increase in PWHT temperature. 8 refs., 6 figs.

A matched chirp transform (MCT) method for detecting a dispersive electromagnetic pulse is described. The unique feature of this transform is that it gives a distribution of signal amplitude over time rather than frequency, thereby simplifying signal detection and identification in the case described here. In the MCT method, the incoming signal is matched to a set of signal segments that chirp in accordance with an expected model of the dispersive medium. The performance of the MCT method is compared to that of a standard periodogram method of frequency measurement.

In previous RADLAC-II beam propagation experiments, stable propagation over a Nordsieck length, in full pressure Albuquerque air (p {approximately}640 Torr) was observed. In these experiments, high transverse momentum resulted in a large equilibrium radius and thus a long betatron wavelength. Following the completion of the RADLAC-II upgrade, a new set of experiments with a small diameter (d {approximately}2 cm), high current (I {approximately}40 kA), low transverse momentum ({beta}{perpendicular} {approximately}0.2) should be possible. The development of time-resolved diagnostics, data analysis codes, and the formulation of output from theoretical calculations in a format as seen by these diagnostics in the lab continues to be a major source of effort in the program. 2 figs.

The final link in the High-Power Microwave (HPM) coupling chain is the distribution of energy on printed-circuit (pc) boards. This distribution is a critical part of the total problem, because the bottom line for damage or upset is what occurs at the component level. Like ports-of-entry (POE's), board coupling paths have their own transfer functions. Since most pc boards are not designed to operate at microwave frequencies, these transfer functions can be very complicated. In addition, active elements on the board are likely to make this part of the problem non-linear. 3 refs., 5 figs.

This paper reports the changes caused by fast neutrons and 200 MeV protons in the electrical properties of high electron mobility transistors (HEMT). A larger gate voltage was required after irradiation with neutron fluences in the 1E14 to 2E15 n/cm{sup 2} range and 200 MeV proton fluences in the 1E14 to 1E15 p/cm{sup 2} range than was required prior to irradiation to obtain the same value of I{sub ds}. The increase in gate voltage required to compensate for a fluence of 1E15 protons/cm{sup 2} was up to four times as great as that required to compensate for the same fluence of neutrons. All devices showed microwave gain (s21) after exposure to 6E14 particles/cm{sup 2} if the gate bias was adjusted to maintain the pre-irradiation value of I{sub ds}. Gamma irradiation at 5E7 rads(GaAs) had no detectable effect on the devices. 8 refs., 6 figs., 1 tab.

Concerns about low-{gamma} relativistic electron beams (REB) being initially injected into the RLA and about energy spreads due to degradation of the accelerating cavity repeating pulse shapes have resulted in our designing a new 4-MV, 20-kA injector, improving the 24-switch trigger system for the ET-2 cavity, and identifying critical factors in the cavity design that affect the pulse shape. We summarize the Metglas inductively isolated, stacked cavity injector design and report on the improvements (completed and proposed) for the ET-2 cavity pulsed power. 7 refs., 6 figs.

Three prototype zinc/bromine batteries were evaluated a Sandia during the last year. The objectives of these tests were to determine performance, cycle life, durability of the auxiliary components, and failure mechanisms. All three were deliverables from a Sandia development contract with Energy Research Corporation (ERC). The test results were communicated to ERC along with suggestions for improving battery design and reliability. 3 figs., 2 tabs.

Zinc/bromine flow batteries are being developed for vehicular and utility load leveling applications by Johnson Controls Co. and Energy Research Corp. under DOE sponsorship. Problems that have been encountered with the zinc/bromine battery are loss of coulombic efficiency brought about by permeation of bromine through the separator and limited life caused by attack of the bromine-containing electrolyte on plastic parts, particularly the flow frame. In this paper, we show that large decreases in the bromine transport rates through microporous separators can be achieved with only a minimal loss of conductivity and identify a chemically stable replacement for PVC, a flowframe material. 4 figs., 1 tab.

The working group on electrical breakdown in vacuum was charged with considering all possible mechanisms by which electrical breakdown might occur either through the vacuum or along insulator bushings in large area electron beam emitter assemblies. It was understood that present systems need to be scaled up, by an order of magnitude or more in both beam area and total energy, to meet demands for higher power and larger size machines, and that increases in the e-beam current density and transport efficiency are also sought. A consideration of the consequences of such a scale-up was pertinent to many of the topics listed in the working-group agenda. Our group attempted to address each of these topics. 18 refs.

Whenever a new elastomer is formulated or an old formulation is modified, it is important to estimate the material's anticipated lifetime in various use environments. For extended lifetimes (years) this often requires the application of accelerated aging techniques which typically involve the modelling of results obtained at higher-than-ambient environmental stress levels. For many practical applications of elastomers, air is present during environmental exposures -- this usually implies that important oxidation effects underly the degradation of the material. Unfortunately, exposure of elastomers to air during aging often results in inhomogeneously oxidized samples, a complication which impacts attempts both to understand the oxidation process and to extrapolate accelerated exposures to long-term conditions. As has been clear for many years, in order to confidently extrapolate shorter-term accelerated simulations to long-term, air-aging conditions, one must be able to monitor and quantitatively understand diffusion-limited oxidation effects. In this review we will highlight some of the recent developments in both experimental techniques and theoretical modelling of relevance to this goal. 28 refs., 12 figs.

The discrete ordinates (S{sub N}) method, first developed for stellar atmospheres, has been used extensively on various other radiation transport problems. In reactor analysis the method is generally used to generate parameters for design models based on more approximate but less expensive methods (such as diffusion theory) so that the spatial-spectrum coupling is represented accurately on a microscopic reaction rate level. It has a decisive advantage over Monte Carlo methods in computing the pin and assembly power profiles. In shielding problems where the penetration of the radiation can be deep, the method is used widely in design calculations. In oil-well logging problems which also involve deep penetration and have a stringent accuracy requirement on the detector responses, the method complements the Monte Carlo techniques. Recently, the discrete ordinates method with appropriate cross sections has been used in coupled photon-electron transport problems. In this paper the basic method is briefly reviewed, its applications illustrated, its merits and pitfalls discussed, and the recent advances in the attendant numerical techniques which have enhanced the capabilities of the method are enumerated. 28 refs., 1 fig.

During severe light water reactor accidents like Three-Mile Island (TMI-2), the reactor core can suffer considerable damage. Of interest here are melt progression, oxidation and gas phase natural convection in the reactor core after the fuel rods suffer a significant loss of geometry. This study describes a two-dimensional porous medium model that considers the motion of three fields: vapor, melt, and solid. A base case solution is described and the effects of oxidation, melt relocation, and Fe-Zr interactions are discussed. 16 refs., 7 figs.

Materials Control techniques are utilized to provide assurance that nuclear materials are being handled properly. In the event that materials are improperly handled or potentially malevolent activities utilizing nuclear materials are initiated, the materials control approach should provide a real-time indication to allow a rapid mitigating response. The appropriate response can range from correcting an inadvertent error to preventing an intentional insider-perpetrated incident. This paper is directed at the use of materials control techniques to deter and detect insider malevolence. 1 fig.

A two-part polyurethane foam has been tested in the laboratory and in the field to assess its utility in controlling lost circulation encountered when drilling geothermal wells. A field test was conducted in The Geysers in January, 1988, to evaluate the chemical formulation and downhole tool used to deploy the chemicals. Although the tool apparently functioned properly in the field test, the chemicals failed to expand sufficiently downhole, instead forming a dense polymer that may be ineffective in sealing loss zones. Subsequent laboratory tests conducted under simulated downhole conditions indicate that the foam chemical undergo sever mixing with water in the wellbore, which disturbs the kinetics of the chemical reaction more than was previously contemplated. The results indicate that without significant changes in the foam chemical formulation or delivery technique, the foam system will be ineffective in lost circulation control except under very favorable conditions. 4 refs., 6 figs., 2 tabs.

Results of fixed-bed hydropyrolysis and low temperature hydrogenation tests with a selection of coals and dispersed catalysts are described. Tar yields greater than 60% have been achieved in hydropyrolysis using sulphided molybdenum (Mo) with Mo concentrations as low as 0.1% daf coal for a number of bituminous coals. The hydrogenation tests indicated that the threshold temperature with these catalysts for oil generation from bituminous coals is 350{degree}C. 16 refs., 2 figs., 2 tabs.

We have developed a fast parallel version of an existing synthetic aperture radar (SAR) simulation program, SRIM. On a 1024-processor NCUBE hypercube it runs an order of magnitude faster than on a CRAY X-MP or CRAY Y-MP processor. This speed advantage is coupled with an order of magnitude advantage in machine acquisition cost. SRIM is a somewhat large (30,000 lines of Fortran 77) program designed for uniprocessors; its restructuring for hypercube provides new lessons in the task of altering older serial programs to run well on modern parallel architectures. We describe the techniques used for parallelization, and the performance obtained. Several novel parallel approaches to problems of task distribution, and direct output were required. These techniques increase performance and appear to have general applicability for massive parallelism. We describe the hierarchy necessary to dynamically manage (i.e., load balance) a large ensemble. The ensemble is used in a heterogeneous manner, with different programs on different parts of the hypercube. The heterogeneous approach takes advantage of the independent instruction streams possible on MIMD machines. 18 refs., 7 figs., 4 tabs.

The Buckshot code is a gridless particle simulation code which is used extensively at Sandia to study relativistic electron beam propagation in the ion-focused regime. The present version of the code evaluates the force on a particle by summing over all the other particles, thus the execution time is proportional to N{sup 2} where N is the number of simulation particles. A new gridless field solver has been developed with time scaling of N log N and the breakeven point between the old and new code is around N = 64 on the Cray X-MP computer. For N = 1000, the new solver is about nine times faster than the old version. The new solver is based on a solution of the two-dimensional Poisson equation which if Fourier decomposed in the azimuthal direction and the solution of the radial equation is represented by integrals over the charge density. These integrals are then replaced by sums over the simulation particles which are assumed to be point particles. The near-field singularity is removed by the Fourier decomposition so long as the number of Fourier modes is much less than the number of simulation particles. The algorithm is written in such a way that the field due to a given species is Fourier decomposed with respect to the center of mass of that species, thus it is possible to study linear and nonlinear ion hose physics with a very small number of azimuthal modes. Typically M = 2 is found to be sufficient for most IFR problems. The old and new solvers have been compared and the agreement is excellent. 2 refs., 3 figs.

It has been shown that a constant axial magnetic field does not affect the growth rate of the ion hose instability. However, if the field is allowed to vary in time, on the ion motion time scale, it is expected that particle orbits will be affected in a way that will result in a time varying beam wavelength. This can lead to detuning of the instability. Results of the rigid model with a time varying field of strength similar to the channel strength, show a significant decrease in the growth of the instability. Also, simulations using the BUCKSHOT code confirm the small effect of a steady magnetic field on hose growth and show a significant decrease in growth with a time varying field. 3 figs.

Sandia National Laboratories (SNL) has been involved in the evaluation of the sodium/sulfur technology for several years. Until recently, the effort concentrated on the performance of single cells. Recently, the evaluation of 4-cell string was initiated. The majority of the activity during the past two years has focused on cells from Chloride Silent Power, Limited (CSPL). To date, four groups of PB cells and 4-cell strings, which consisted of PB cells, have been evaluated. The first group of ten cells delivered to Sandia were on test for approximately one year. The majority of these cells failed due to corrosion problems in the sulfur seal. However, two cells completed over 800 cycles, and one of these cells completed nearly 1600 cycles. 4 figs., 1 tab.

A high detectivity infrared photodiode was constructed using an InAs{sub 0.15}Sb{sub 0.85}/InSb strained-layer superlattice (SLS). The surface passivated device exhibited detectivities {ge} 1 {times} 10{sup 10} cm{radical}Hz/W at wavelengths {le} 10 {mu}m. This device demonstrates the feasibility of a long wavelength, photovoltaic infrared detector technology based on InAsSb SLSs. 8 refs., 4 figs.