Direct Observation of an Abrupt Insulator-to-Metal Transition in Dense Liquid Deuterium
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Journal of Applied Physics
Magnetically-driven, planar shockless-compression experiments to multi-megabar pressures were performed on tantalum samples using a stripline target geometry. Free-surface velocity waveforms were measured in 15 cases; nine of these in a dual-sample configuration with two samples of different thicknesses on opposing electrodes, and six in a single-sample configuration with a bare electrode opposite the sample. Details are given on the application of inverse Lagrangian analysis (ILA) to these data, including potential sources of error. The most significant source of systematic error, particularly for single-sample experiments, was found to arise from the pulse-shape dependent free-surface reflected wave interactions with the deviatoric-stress response of tantalum. This could cause local, possibly temporary, unloading of material from a ramp compressed state, and thus multi-value response in wave speed that invalidates the free-surface to in-material velocity mapping step of ILA. By averaging all 15 data sets, a final result for the principal quasi-isentrope of tantalum in stress-strain was obtained to a peak longitudinal stress of 330GPa with conservative uncertainty bounds of ±4.5% in stress. The result agrees well with a tabular equation of state developed at Los Alamos National Laboratory.
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Temperature measurements are very important in shock and ramp type dynamic materials experiments. In particular, accurate temperature measurements can provide stringent additional constraints on determining the equation of state for materials at high pressure. The key to providing these constraints is to develop diagnostic techniques that can determine the temperature with sufficient accuracy. To enable such measurements, we are working to improve our diagnostic capability with three separate techniques, each of which has specific applicability in a particular temperature range. To improve our capability at low temperatures (< 1 eV) we are working on a technique that takes advantage of the change in reflectivity of Au as the temperature is increased. This is most applicable to ramp type experiments. In the intermediate range (~1 eV < T< 5-10 eV) we are improving our optical pyrometry diagnostic by adding the capability of doing an absolute calibration as part of the diagnostic procedure for the shock or shock ramp dynamic materials experiment. This will enable more accurate temperature measurements for shock and shock ramp type experiments. For higher temperatures that occur in very high-pressure shock experiments, above 10 eV, we are developing the capability of doing x-ray Thomson scattering measurements. Such measurements will enable us to characterize strongly shocked or warm dense matter materials. Work on these diagnostic approaches is summarized in this report.
S hock compression exper iments in the few hundred GPa (multi - Mabr) regime were performed on Lithium Deuteride (LiD) single crystals . This study utilized the high velocity flyer plate capability of the Sandia Z Machine to perform impact experiments at flyer plate velocities in the range of 17 - 32 km/s. Measurements included pressure, density, and temperature between %7E200 - 600 GPa along the Principal Hugoniot - the locus of end states achievable through compression by large amplitude shock waves - as well as pressure and density of re - shock states up to %7E900 GPa . The experimental measurements are compared with recent density functional theory calculations as well as a new tabular equation of state developed at Los Alamos National Labs.
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Nature
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Physical Review Applied
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Journal of Physics: Conference Series
In this article we discuss scaling the magnetically accelerated flyer plate technique to currents greater than is available on the Z accelerator. Peak flyer plate speeds in the range 7-46 km/s are achieved in pulsed power driven, hyper-velocity impact experiments on Z for peak currents in the range 8-20 MA. The highest (lowest) speeds are produced using aluminum (aluminum-copper) flyer plates. In either case, the ≈1 mm thick flyer plate is shocklessly accelerated by magnetic pressure to ballistic speed in ≈400 ns; it arrives at the target with a fraction of material at standard density. During acceleration a melt front, due to resistive heating, moves from the drive-side toward the target-side of the flyer plate; the speed of the melt front increases with increasing current. Peak flyer speeds on Z scale quadratically (linearly) with current at the low (high) end of the range. Magnetohydrodynamic simulation shows that the change in scaling is due to geometric deformation, and that linear scaling continues as current increases. However, the combined effects of shockless acceleration and resistive heating lead to an upper bound on the magnetic field feasible for pulsed power driven flyer plate experiments, which limits the maximum possible speed of a useful flyer plate to < 100 km/s. © Published under licence by IOP Publishing Ltd.
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