Thermal-Mechanical Data of Argillite and Crystalline Disposal Systems: A First-Principles Approach
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Inorganic Chemistry
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Inorganic Chemistry
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Report RWEV-REP-001, Analysis of Postclosure Groundwater Impacts for a Geologic Repository for the Disposal of Spent Nuclear Fuel and High Level Radioactive Waste at Yucca Mountain, Nye County, Nevada was issued by the DOE in 2009 and is currently being updated. Sandia National Laboratories (SNL) provided support for the original document, performing calculations and extracting data from the Yucca Mountain Performance Assessment Model that were used as inputs to the contaminant transport and dose calculations by Jason Associates Corporation, the primary developers of the DOE report. The inputs from SNL were documented in LSA-AR-037, Inputs to Jason Associates Corporation in Support of the Postclosure Repository Supplemental Environmental Impact Statement. To support the updating of the original Groundwater Impacts document, SNL has reviewed the inputs provided in LSA-AR-037 to verify that they are current and appropriate for use. The results of that assessment are documented here.
Journal of Physical Chemistry C
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14th International High-Level Radioactive Waste Management Conference, IHLRWMC 2013: Integrating Storage, Transportation, and Disposal
Within the Used Fuel Disposition Campaign (UFDC) of the United States Department of Energy Office of Nuclear Energy (DOE-NE), we have investigated used fuel (UF) degradation and radionuclide mobilization (UFD&RM) and implemented/produced a set of models encompassing radiolytic processes, UF matrix degradation, instant release fractions (IRF) of key radionuclides, and first-principles atomistic models for UO2 and its potential corrosion products. The goals of this collaborative effort (among three different national laboratories: Argonne National Laboratory [ANL]; Pacific Northwest National Laboratory [PNNLJ; and Sandia National Laboratories [SNL]) are to enhance the understanding of UF degradation processes and the technical bases for safety analyses in a range of generic disposal environments. In addition to these modeling efforts, integrated experimental studies are being conducted at both ANL and PNNL to evaluate and validate (and ultimately expand) process models for radiolytic phenomena and UF matrix degradation in various geologic disposal conditions. Integration and coupling of these process models into a generic performance assessment model (GPAM) is one focus of SNL efforts within the generic analyses of the Engineered Barrier System (EBS) for various repository environments. As discussed below, the present work has produced a set of models for implementation into the GPAM as an initial step towards an enhanced coupled model of source-term processes.
Physics Review Lettters
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Journal of the Electrochemical Society
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Journal of the American Chemical Society
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Geochimica et Cosmochimica Acta
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European Journal of Inorganic Chemistry
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Proposed for publication in European Journal of Inorganic Chemistry.
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Proposed for publication in Inorganic Chemistry.
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Proposed for publication in J. Am. Chem. Soc.
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Proposed for publication in Dalton Transactions.
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Proposed for publication in J. Am. Chem. Soc..
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Proposed for publication in Inorganic Chemistry.
Abstract not provided.