Publications

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It has been predicted that several changes will occur when premixed flames are subjected to the extreme levels of turbulence that can be found in practical combustors. This paper is a review of recent experimental and DNS results that have been obtained for the range of extreme turbulence, and it includes a discussion of cases that agree or disagree with predictions. “Extreme turbulence” is defined to correspond to a turbulent Reynolds number (ReΤ, based on integral scale) that exceeds 2800 or a turbulent Karlovitz number that exceeds 100, for reasons that are discussed in Section 2.1. Several data bases are described that include measurements made at Lund University, the University of Sydney, the University of Michigan and the U.S. Air Force Research Lab. The data bases also include DNS results from Sandia National Laboratory, the University of New South Wales, Newcastle University, the California Institute of Technology and the University of Cambridge. Several major observations are: (a) DNS now can be achieved for a realistic geometry (of the Lund University jet burner) even for extreme turbulence levels, (b) state relations (conditional mean profiles) from DNS and experiments do tend to agree with laminar profiles, at least for methane-air and hydrogen-air reactants that are not preheated, and (c) regime boundaries have been measured and they do not agree with predicted boundaries. These findings indicate that the range of conditions for which flamelet models should be valid is larger than what was previously believed. Additional parameters have been shown to be important; for example, broken reactions occur if the “back-support” is insufficient due to the entrainment of cold gas into the product gas. Turbulent burning velocity measurements have been extended from the previous normalized turbulence levels (u’/SL) of 24 up to a value of 163. Turbulent burning velocities no longer follow the trend predicted by Shchelkin but they tend to follow the trend predicted by Damköhler. The boundary where flamelet broadening begins was measured to occur at ReTaylor = 13.8, which corresponds to an integral scale Reynolds number (ReT) of 2800. This measured regime boundary can be explained by the idea that flame structure is altered when the turbulent diffusivity at the Taylor scale exceeds a critical value, rather than the idea that changes occur when Kolmogorov eddies just fit inside a flamelet. A roadmap to extend DNS to complex chemistry and to higher Reynolds numbers is discussed. Exascale computers, machine learning, adaptive mesh refinement and embedded DNS show promise. Some advances are reviewed that have extended the use of line and planar PLIF and CARS laser diagnostics to studies that consider complex hydrocarbon fuels and harsh environments.

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The ignition process in diesel engines is highly complex and incompletely understood. In the present study, two-dimensional direct numerical simulations are performed to investigate the ignition dynamics and their sensitivity to thermochemical and mixing parameters. The thermochemical and mixing conditions are matched to the benchmark Spray A experiment from the Engine Combustion Network. The results reveal a complex ignition process with overlapping stages of: low-temperature ignition (cool flames), rich premixed ignition, and nonpremixed ignition, which are qualitatively consistent with prior experimental and numerical investigations, however, this is the first time that fully-resolved simulations have been reported at the actual Spray A thermochemical condition. Parametric variations are then performed for the Damkohler number Da, oxidiser temperature, oxygen concentration, and peak mixture fraction (a measure of premixedness), to study their effect on the ignition dynamics. It is observed that with both increasing oxidiser temperature and decreasing oxygen concentration, that the cool flame moves to richer mixtures, the overlap in the ignition stages decreases, and the (nondimensional) time taken to reach a fully burning state increases. With increasing Da, the cool-flame speed is decreased due to lower mean mixing rates, which causes a delayed onset of high-temperature ignition. With increasing peak mixture fraction, the onset of each stage of ignition is not affected, but the overall duration of the ignition increases leading to a longer burn duration. Overall, the results suggest that turbulence-chemistry interactions play a significant role in determining the timing and location in composition space of the entire ignition process.

The link between the distribution of fluid residence time and the distribution of reactive scalars is analysed using Direct Numerical Simulation data. Information about the reactive scalar distribution is needed in order to model the reaction terms that appear in Large Eddy and Reynolds-Averaged simulations of turbulent reacting flows. The lifted flame is simulated taking account of multi-step chemistry for dimethyl-ether fuel. Due to autoignition and flame propagation, the reaction progress increases with residence time. The variation of fluid residence time is evaluated by solving an Eulerian transport equation for the fluid age. The fluid age is a passive scalar with a spatially-uniform source term, meaning that its moments and dissipation rates in turbulent flows can be modelled using closures already established for conserved scalars such as mixture fraction. In combination with the mixture fraction, the fluid age serves as a useful mapping variable to distinguish younger less-reacted fluid near the inlet from older more-reacted fluid downstream. The local fluctuations of mixture fraction and fluid age have strong negative correlation and, building upon established presumed-pdf models for mixture fraction, this feature can be used to construct an accurate presumed-pdf model for the joint mixture fraction/fluid age pdf. It is demonstrated that the double-conditional first-order moment closure combined with the proposed presumed model for the joint pdf of mixture fraction and fluid age gives accurate predictions for unconditional reaction rates - both for pre-ignition radical species produced by low-temperature processes upstream of the flame base, and for major species that are produced at the flame front.

A three-dimensional direct numerical simulation (DNS) is performed for a turbulent hydrogen-air flame, represented with detailed chemistry, stabilized in a model gas-turbine combustor. The combustor geometry consists of a mixing duct followed by a sudden expansion and a combustion chamber, which represents a geometrically simplified version of Ansaldo Energia's GT26/GT36 sequential combustor design. In this configuration, a very lean blend of hydrogen and vitiated air is prepared in the mixing duct and convected into the combustion chamber, where the residence time from the inlet of the mixing duct to the combustion chamber is designed to coincide with the ignition delay time of the mixture. The results show that when the flame is stabilized at its design position, combustion occurs due to both autoignition and flame propagation (deflagration) modes at different locations within the combustion chamber. A chemical explosive mode analysis (CEMA) reveals that most of the fuel is consumed due to autoignition in the bulk-flow along the centerline of the combustor, and lower amounts of fuel are consumed by flame propagation near the corners of the sudden expansion, where the unburnt temperature is reduced by the thermal wall boundary layers. An unstable operating condition is also identified, wherein periodic auto-ignition events occur within the mixing duct. These events appear upstream of the intended stabilization position, due to positive temperature fluctuations induced by pressure waves originating from within the combustion chamber. The present DNS investigation represents the initial step of a comprehensive research effort aimed at gaining detailed physical insight into the rate-limiting processes that govern the sequential combustor behavior and avoid the insurgence of the off-design auto-ignition events.

Laminar natural gas flames are investigated at engine-relevant thermochemical conditions where the ignition delay time τ is short due to very high ambient temperatures and pressures. At these conditions, it is not possible to measure or calculate well-defined values for the laminar flame speed s_l, laminar flame thickness δ_l, and laminar flame time scale ${\tau }_l={\delta }_l/s_l$ due to the explosive thermochemical state. The corresponding reference values, s_R, δ_R, and ${\tau }_R={\delta }_R/s_R,$ that account for the effects of autoignition, are numerically estimated to investigate the enhancement of flame propagation, and the competition with autoignition that arises under nominally autoignitive conditions (characterised here by the number τ/τ_R). Large values of τ/τ_R indicate that autoignition is unimportant, values near or below unity indicate that flame propagation is not possible, and intermediate values indicate that a combination of both flame propagation and autoignition may be important, depending upon factors such as device geometry, turbulence, stratification, et cetera. The reference quantities are presented for a wide range of temperatures, equivalence ratios, pressures, and hydrogen concentrations, which includes conditions relevant to stationary gas turbine reheat burners and boosted spark ignition engines. It is demonstrated that the transition from flame propagation to autoignition is only dependent on residence time, when the results are non-dimensionalised by the reference values. The temporal evolution of the reference values are also reported for a modelled boosted SI engine. It is shown that the nominally autoignitive conditions enhance flame propagation, which may be an ameliorating factor for the onset of engine knock. The calculations are performed using a recently-developed, detailed 177 species mechanism for C0–C3 chemistry that is derived from theoretical chemistry and is suitable for a wide range of thermochemical conditions as it is not tuned or optimised for a particular operating condition.

Direct numerical simulations are performed to investigate the transient upstream flame propagation (flashback) through homogeneous and fuel-stratified hydrogen-air mixtures transported in fully developed turbulent channel flows. Results indicate that, for both cases, the flame maintains steady propagation against the bulk flow direction, and the global flame shape and the local flame characteristics are both affected by the occurrence of fuel stratification. Globally, the mean flame shape undergoes an abrupt change when the approaching reactants transition from an homogeneous to a stratified mixing configuration. A V-shaped flame surface, whose leading-edge is located in the near-wall region, characterizes the nonstratified, homogeneous mixture case, while a U-shaped flame surface, whose leading edge propagates upstream at the channel centerline, distinguishes the case with fuel stratification (fuel-lean in the near-wall region and fuel-rich away from the wall). The characteristic thickness, wrinkling, and displacement speed of the turbulent flame brush are subject to considerable changes across the channel due to the dependence of the turbulence and mixture properties on the distance from the channel walls. More specifically, the flame transitions from a moderately wrinkled, thin-flamelet combustion regime in the homogeneous mixture case to a strongly wrinkled flame brush more representative of a thickened-flame combustion regime in the near-wall region of the fuel-stratified case. The combustion regime may be related to the Karlovitz number, and it is shown that a nominal channel-flow Karlovitz number, Kainch, based on the wall-normal variation of canonical turbulence (tη=(ν/ϵ)1/2) and chemistry (tl=δl/Sl) timescales in fully developed channel flow, compares well with an effective Karlovitz number, Kaflch, extracted from the present DNS datasets using conditionally sampled values of tη and tl in the immediate vicinity of the flame (0.1

We present a direct numerical simulation of a temporal jet between n-dodecane and diluted air undergoing spontaneous ignition at conditions relevant to low-temperature diesel combustion. The jet thermochemical conditions were selected to result in two-stage ignition. Reaction rates were computed using a 35-species reduced mechanism which included both the low- and high-temperature reaction pathways. The aim of this study is to elucidate the mechanisms by which low-temperature reactions promote high-temperature ignition under turbulent, non-premixed conditions. We show that low-temperature heat release in slightly rich fuel regions initiates multiple cool flame kernels that propagate towards very rich fuel regions through a reaction-diffusion mechanism. Although low-temperature ignition is delayed by imperfect mixing, the propagation speed of the cool flames is high: as a consequence, high-temperature reactions in fuel-rich regions become active early during the ignition transient. Because of this early start, high-temperature ignition, which occurs in fuel-rich regions, is faster than homogeneous ignition. Following ignition, the high-temperature kernels expand and engulf the stoichiometric mixture-fraction iso-surface which in turn establish edge flames which propagate along the iso-surface. The present results indicate the preponderance of flame folding of existing burning surfaces, and that ignition due to edge-flame propagation is of lesser importance. Finally, a combustion mode analysis that extends an earlier classification [1] is proposed to conceptualize the multi-stage and multi-mode nature of diesel combustion and to provide a framework for reasoning about the effects of different ambient conditions on diesel combustion.

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