The Neutron Scatter Camera (NSC) is a neutron spectrometer and imager that has been developed and improved by the Sandia National Laboratories for several years. Built for special nuclear material searches, the instrument was configured by the design to reconstruct neutron sources within the fission energy range 1–10 MeV. In this work, we present modifications that attempt to extend the NSC sensitivity to neutron energies in the range ~10–200 MeV and discuss the corresponding consequences for the event processing. We present simulation results that manifest important aspects of the NSC response to those intermediate energy neutrons. The simulation results also evidence that the instrument’s spectroscopic capabilities severely deteriorate at those energies, mainly due to the uncertainties in measuring energy, time, and distance between the two neutron scattering interactions. Furthermore, this work is motivated by the need to characterize neutron fluxes at particle accelerators as they may represent important backgrounds for neutrino experiments.
We report on the position, timing, and energy resolution of a range of plastic scintillator bars and reflector treatments using dual-ended silicon photomultiplier readout. These measurements are motivated by the upcoming construction of an optically segmented single-volume neutron scatter camera, in which neutron elastic scattering off of hydrogen is used to kinematically reconstruct the location and energy of a neutron-emitting source. For this application, interaction position resolutions of about 10 mm and timing resolutions of about 1 ns are necessary to achieve the desired efficiency for fission-energy neutrons. The results presented here indicate that this is achievable with an array of 5×5×190mm 3 bars of EJ-204 scintillator wrapped in Teflon tape, read out with SensL's J-series 6×6mm 2 silicon photomultipliers. With two independent setups, we also explore the systematic variability of the position resolution, and show that, in general, using the difference in the pulse arrival time at the two ends is less susceptible to systematic variation than using the log ratio of the charge amplitude of the two ends. Finally, we measure a bias in the absolute time of interactions as a function of position along the bar: the measured interaction time for events at the center of the bar is ∼100 ps later than interactions near the SiPM.
The development of fast, highly pixelated photodetectors with single-photon sensitivity has the potential to enable a variety of new radiation detection concepts. Systems that desire to employ these detectors without loss of information demand waveform digitization with high sampling rates. Switched capacitor arrays provide a low-cost, low-power, compact solution to fast readout with high channel density. The Sandia Laboratories Compact Electronics for Modular Acquisition (SCEMA) was developed to meet these demands. A single module employs two domino ring sampling switched capacitor arrays (DRS4) [1] to provide 16 channels of up to 5 GS/s waveform digitization. This paper presents an overview of the board design and function. Calibration procedures for the module are discussed. Finally, temporal resolution tests are presented demonstrating the module's viability as readout for high fidelity temporal measurements of single photons in suitable photodetectors.
The scintillation anisotropy effect for proton recoil events has been investigated in five pure organic crystalline materials: Anthracene, trans-stilbene, p-terphenyl, bibenzyl, and diphenylacetylene (DPAC). These measurements include the characterization of the scintillation response for one hemisphere of proton recoil directions in each crystal. In addition to standard measurements of the total light output and pulse shape at each angle, the prompt and delayed light anisotropies are analyzed, allowing for the investigation of the singlet and triplet molecular excitation behaviors independently. This paper provides new quantitative and qualitative observations that make progress toward understanding the physical mechanisms behind the scintillation anisotropy. These measurements show that the relationship between the prompt and delayed light anisotropies is correlated with a crystal structure, as it changes between the pi-stacked crystal structure materials (anthracene and p-terphenyl) and the herringbone crystal structure materials (stilbene, bibenzyl, and DPAC). The observations are consistent with a model in which there are preferred directions of kinetic processes for the molecular excitations. These processes and the impact of their directional dependences on the scintillation anisotropy are discussed.
This paper presents the model-based design and evaluation of an instrument that estimates incident neutron direction using the kinematics of neutron scattering by hydrogen-1 nuclei in an organic scintillator. The instrument design uses a single, nearly contiguous volume of organic scintillator that is internally subdivided only as necessary to create optically isolated pillars, i.e., long, narrow parallelepipeds of organic scintillator. Scintillation light emitted in a given pillar is confined to that pillar by a combination of total internal reflection and a specular reflector applied to the four sides of the pillar transverse to its long axis. The scintillation light is collected at each end of the pillar using a photodetector, e.g., a microchannel plate photomultiplier (MCP-PM) or a silicon photomultiplier (SiPM). In this optically segmented design, the (x,y) position of scintillation light emission (where the x and y coordinates are transverse to the long axis of the pillars) is estimated as the pillar's (x,y) position in the scintillator “block”, and the z-position (the position along the pillar's long axis) is estimated from the amplitude and relative timing of the signals produced by the photodetectors at each end of the pillar. The neutron's incident direction and energy is estimated from the (x,y,z)-positions of two sequential neutron–proton scattering interactions in the scintillator block using elastic scatter kinematics. For proton recoils greater than 1 MeV, we show that the (x,y,z)-position of neutron–proton scattering can be estimated with < 1 cm root-mean-squared [RMS] error and the proton recoil energy can be estimated with < 50 keV RMS error by fitting the photodetectors’ response time history to models of optical photon transport within the scintillator pillars. Finally, we evaluate several alternative designs of this proposed single-volume scatter camera made of pillars of plastic scintillator (SVSC-PiPS), studying the effect of pillar dimensions, scintillator material (EJ-204, EJ-232Q and stilbene), and photodetector (MCP-PM vs. SiPM) response vs. time. We demonstrate that the most precise estimates of incident neutron direction and energy can be obtained using a combination of scintillator material with high luminosity and a photodetector with a narrow impulse response. Specifically, we conclude that an SVSC-PiPS constructed using EJ-204 (a high luminosity plastic scintillator) and an MCP-PM will produce the most precise estimates of incident neutron direction and energy.
We present the design, characterization, and testing of a laboratory prototype radiological search and localization system. The system, based on time-encoded imaging, uses the attenuation signature of neutrons in time, induced by the geometrical layout and motion of the system. We have demonstrated the ability to detect a ∼1mCi252Cf radiological source at 100m standoff with 90% detection efficiency and 10% false positives against background in 12min. This same detection efficiency is met at 15s for a 40m standoff, and 1.2s for a 20m standoff.
We investigate the feasibility of constructing a data-driven distance metric for use in null-hypothesis testing in the context of arms-control treaty verification. The distance metric is used in testing the hypothesis that the available data are representative of a certain object or otherwise, as opposed to binary-classification tasks studied previously. The metric, being of strictly quadratic form, is essentially computed using projections of the data onto a set of optimal vectors. These projections can be accumulated in list mode. The relatively low number of projections hampers the possible reconstruction of the object and subsequently the access to sensitive information. The projection vectors that channelize the data are optimal in capturing the Mahalanobis squared distance of the data associated with a given object under varying nuisance parameters. The vectors are also chosen such that the resulting metric is insensitive to the difference between the trusted object and another object that is deemed to contain sensitive information. Data used in this study were generated using the GEANT4 toolkit to model gamma transport using a Monte Carlo method. For numerical illustration, the methodology is applied to synthetic data obtained using custom models for plutonium inspection objects. The resulting metric based on a relatively low number of channels shows moderate agreement with the Mahalanobis distance metric for the trusted object but enabling a capability to obscure sensitive information.
This paper reports a series of measurements that characterize the directional dependence of the scintillation response of crystalline melt-grown and solution-grown trans-stilbene to incident DT and DD neutrons. These measurements give the amplitude and pulse shape dependence on the proton recoil direction over one hemisphere of the crystal, confirming and extending previous results in the literature for melt-grown stilbene and providing the first measurements for solution-grown stilbene. In similar measurements of liquid and plastic detectors, no directional dependence was observed, confirming the hypothesis that the anisotropy in stilbene and other organic crystal scintillators is a result of internal effects due to the molecular or crystal structure and not an external effect on the measurement system.
In an effort to characterize the fast neutron radiation background, 16 EJ-309 liquid scintillator cells were installed in the Radiological Multi-sensor Analysis Platform (RadMAP) to collect data in the San Francisco Bay Area. Each fast neutron event was associated with specific weather metrics (pressure, temperature, absolute humidity) and GPS coordinates. The expected exponential dependence of the fast neutron count rate on atmospheric pressure was demonstrated and event rates were subsequently adjusted given the measured pressure at the time of detection. Pressure adjusted data was also used to investigate the influence of other environmental conditions on the neutron background rate. Using National Oceanic and Atmospheric Administration (NOAA) coastal area lidar data, an algorithm was implemented to approximate sky-view factors (the total fraction of visible sky) for points along RadMAPs route. Three areas analyzed in San Francisco, Downtown Oakland, and Berkeley all demonstrated a suppression in the background rate of over 50% for the range of sky-view factors measured. This effect, which is due to the shielding of cosmic-ray produced neutrons by surrounding buildings, was comparable to the pressure influence which yielded a 32% suppression in the count rate over the range of pressures measured.