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Time-resolved picosecond pure-rotational coherent anti-stokes Raman spectroscopy for thermometry and species concentration in flames

Kliewer, Christopher; Farrow, Roger L.; Settersten, Thomas B.; Kiefer, Johannes; Patterson, Brian; Gao, Yi; Settersten, Thomas B.

Time-resolved picosecond pure-rotational coherent anti-Stokes Raman spectroscopy is demonstrated for thermometry and species concentration determination in flames. Time-delaying the probe pulse enables successful suppression of unwanted signals. A theoretical model is under development. ©2010 Optical Society of America.