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Radiation embrittlement of the neutron shield tank from the Shippingport reactor

Rosinski, S.T.

The irradiation embrittlement of neutron shield tank (NST) material (A212 Grade B steel) from the Shippingport reactor has been characterized. Irradiation increases the Charpy transition temperature (CTT) by 23--28{degrees}C (41--50{degrees}F) and decreases the upper-shelf energy. The shift in CTT is not as severe as that observed in high-flux isotope reactor (HFIR) surveillance specimens. However, the actual value of the CTT is higher than that for the HFIR data. The increase in yield stress is 51 MPa (7.4 ksi), which is comparable to HFIR data. The NST material is weaker in the transverse orientation than in the longitudinal orientation. Some effects of position across the thickness of the wall are also observed; the CTT shift is slightly greater for specimens from the inner region of the wall. Annealing studies indicate complete recovery from embrittlement after 1 h at 400{degrees}C (752{degrees}F). Although the weld metal is significantly tougher than the base metal, the shifts in CTT are comparable. The shifts in CTT for the Shippingport NST are consistent with the test and Army reactor data for irradiations at <232{degrees}C (<450{degrees}F) and show very good agreement with the results for HFIR A212-B steel irradiated in the Oak Ridge Research Reactor (ORR). The effects of irradiation temperature, fluence rate, and neutron flux spectrum are discussed. The results indicate that fluence rate has no effect on radiation embrittlement at rates as low as 2 {times} 10{sup 8} n/cm{sup 2}{center dot}s and at the low operating temperatures of the Shippingport NST, i.e., 55{degrees}C (130{degrees}F). This suggests that the accelerated embrittlement of HFIR surveillance samples is most likely due to the relatively higher proportion of thermal neutrons in the HFIR spectrum compared to that for the test reactors. 28 refs., 25 figs.