Publications Details
Filtration testing for enhanced performance of Radionuclide Monitoring Stations for Nuclear Treaty Verification
A study of aerosol filtration was conducted to improve U.S. Radionuclide Monitoring Station (RMS) performance for Nuclear Treaty Verification. The primary objectives of this study were to improve system operability and maintainability, reduce power consumption and operational cost, and reduce baseline radionuclide sensitivity. To meet these goals, Sandia National Laboratories (SNL) studied the performance of alternate filter materials and aerosol collection technologies that could be engineered into U.S. Radionuclide Monitoring Stations. Laboratory-scale filtration experiments were conducted with Filter Material 1, FM1 (current filter), Filter Material 2, FM2, and Filter Material 3, FM3. All three materials employ electrostatically charged filter fibers to enhance nanoparticle collection. FM2 and FM3 both had higher air permeability with respect to FM1 which is advantageous for high volume collection and power savings. Particle pre-charging, a well-established industrial technique used in electrostatic precipitators, was tested to see if electrostatically charging particles prior to filtration could enhance filter performance. We found that particle-pre-charging did enhance aerosol collection efficiencies for materials which would not have otherwise satisfied RMS performance requirements. Laboratory-scale testing indicated it may be possible to reduce the baseline radionuclide sensitivity to approximately 60% of its current value by increasing the volume of air sampled in 24 hours to 2.5 times the current air volume. Improvements to geolocation may also be possible with shorter air samples (e.g., 12 hours). A new methodology was developed at SNL to assess filter performance using established RMS certification procedures. We coined these tests “mid-scale” since they bridged the gap between laboratory-scale and full-scale RMS testing. Four filter specimens were drawn from the exact same atmospheric aerosol. Gamma spectroscopy was used to assess radiological backgrounds due to radon progeny and other naturally occurring radionuclides. Direct comparisons between the four filters allowed SNL to quantify the relative change in baseline sensitivity by altering air flow rate, filter material, and particle-pre charging. Mid-scale results agreed with laboratory-scale results: alterations to RMS configuration (filter, flow, and particle charge) may result in baseline sensitivities approximately 55-60% of their current values. Finally, an assessment of scalability was performed to determine if technical approaches used in laboratory-scale and mid-scale testing could be engineered into full-scale Radionuclide Monitoring Stations. Results suggested that particle-pre-charging is a viable technical approach if reductions in baseline sensitivity or power consumption are desired.