Publications Details

A-priori analysis of conditional moment closure modeling of turbulent soot formation using direct numerical simulation

Lignell, D.O.; Hewson, J.C.; Chen, J.H.

Modelling soot formation in turbulent nonpremixed combustion is a difficult problem. Unlike most gaseous combustion species, soot lacks a strong state relationship with the mixture fraction due to unsteady formation rates which overlap transport timescales, and strong differential diffusion between gaseous species and soot. The conditional moment closure model (CMC) has recently been applied to the problem of turbulent soot formation. A challenge in CMC modelling is the treatment of differential diffusion. Three-dimensional direct numerical simulation (DNS) of a nonpremixed ethylene jet flame with soot formation has been performed for the first time, using a nineteen species reduced ethylene mechanism and a four-step, three-moment, semi-empirical soot model. The DNS provides full resolution of the turbulent flow field and is used to perform a-priori analysis of a new CMC model derived from the joint scalar PDF transport equation. Unlike other approaches, this CMC model does not require additional transport equations to treat differentially diffusing species. A budget of the terms of the CMC equation for both gaseous species and soot is presented. In particular, exact expressions for unclosed terms are compared to typical closure models for scalar dissipation, cross dissipation, differential diffusion, and reactive source terms.