A growing number of applications involve the transmission of high-intensity laser pulses through optical fibers. Previously, our particular interests led to a series of studies on single-fiber transmission of Q-switched, 1064 nm pulses from multimode Nd:YAG lasers through step-index, multimode, fused silica fibers. The maximum pulse energy that could be transmitted through a given fiber was limited by the onset of laser-induced breakdown or damage. Breakdown at the fiber entrance face was often the first limiting process encountered, but other mechanisms were observed that could result in catastrophic damage at either fiber face, within the initial "entry" segment of the fiber, and at other internal sites along the fiber path. These studies examined system elements that can govern the relative importance of different damage mechanisms, including laser characteristics, the design and alignment of laser-to-flber injection optics, fiber end-face preparation, and fiber routing. In particular, criteria were established for injection optics in order to maximize margins between transmission requirements and thresholds for laser-induced damage. Recent interests have led us to examine laser injection into multiple fibers. Effective methods for generating multiple beams are available, but the resulting beam geometry can lead to challenges in applying the criteria for optimum injection optics. To illustrate these issues, we have examined a three-fiber injection system consisting of a beam-shaping element, a primary injection lens, and a grating beamsplitter. Damage threshold characteristics were established by testing fibers using the injection geometry imposed by this system design.
Shock wave compression of poled Pb{sub 0.99}(Zr{sub 0.95}Ti{sub 0.05}){sub 0.98}Nb{sub 0.02}O{sub 3} (PZT 95/5-2Nb) results in rapid depoling and release of bound charge. In the current study, planar-impact experiments with this material were conducted on a gas-gun facility to determine Hugoniot states, to examine constitutive mechanical properties during shock propagation, and to investigate shock-induced depoling characteristics. A previous article summarized results from the first two of these areas, and this article summarizes the depoling studies. A baseline material, similar to materials used in previous studies, was examined in detail. More limited experiments were conducted with other materials to investigate the effects of different porous microstructures. Experiments were conducted over a wide range of conditions in order to examine the effects of varying shock strength, poling orientation, input wave shape, electric field strength, porous microstructure at a fixed density, and initial density. Depoling currents were recorded in an external circuit under either short-circuit or high-field conditions, and provide a convenient means of examining the kinetics associated with the ferroelectric-to-antiferroelectric phase transition. For sufficiently strong shock waves, the measured short-circuit currents indicate that the phase transition is very rapid and essentially complete. As shock strengths are reduced, short-circuit currents show increasing rise times and decreasing final levels at the end of shock transit. These features indicate that the transition kinetics can be characterized in terms of both a transition rate and a limiting degree of transition achieved in a given shock experiment. The presence of a strong electric field does not appear to have a significant effect on transition kinetics at high shock stresses, but has a strong effect at low stresses. As was found for constitutive mechanical properties, only small effects on measured currents resulted from differences in the porous microstructure of common-density materials, but large effects were observed when initial density was varied. To examine transition kinetics in more detail, short-circuit currents obtained with the baseline material and several approximate methods were used to estimate values for the rate and degree of transition as functions of shock properties. Differences between these currents and currents measured in high-field experiments using the same impact conditions were used to examine field effects on transition kinetics and corresponding dielectric properties.
The particular lead zirconate/titanate composition PZT 95/5-2Nb was identified many years ago as a promising ferroelectric ceramic for use in shock-driven pulsed power supplies. The bulk density and the corresponding porous microstructure of this material can be varied by adding different types and quantities of organic pore formers prior to bisque firing and sintering. Early studies showed that the porous microstructure could have a significant effect on power supply performance, with only a relatively narrow range of densities providing acceptable shock wave response. However, relatively few studies were performed over the years to characterize the shock response of this material, yielding few insights on how microstructural features actually influence the constitutive mechanical, electrical, and phase-transition properties. The goal of the current work was to address these issues through comparative shock wave experiments on PZT 95/5-2Nb materials having different porous microstructures. A gas-gun facility was used to generate uniaxial-strain shock waves in test materials under carefully controlled impact conditions. Reverse-impact experiments were conducted to obtain basic Hugoniot data, and transmitted-wave experiments were conducted to examine both constitutive mechanical properties and shock-driven electrical currents. The present work benefited from a recent study in which a baseline material with a particular microstructure had been examined in detail. This study identified a complex mechanical behavior governed by anomalous compressibility and incomplete phase transformation at low shock amplitudes, and by a relatively slow yielding process at high shock amplitudes. Depoling currents are reduced at low shock stresses due to the incomplete transformation, and are reduced further in the presence of a strong electrical field. At high shock stresses, depoling currents are driven by a wave structure governed by the threshold for dynamic yielding. This wave structure is insensitive to the final wave amplitude, resulting in depoling currents that do not increase with shock amplitude for stresses above the yield threshold. In the present study, experiments were conducted under matched experimental conditions to directly compare with the behavior of the baseline material. Only subtle differences were observed in the mechanical and electrical shock responses of common-density materials having different porous microstructures, but large effects were observed when initial density was varied.
This report summarizes a multiyear effort to establish a new capability for determining dynamic material properties. By utilizing a significant reduction in experimental length and time scales, this new capability addresses both the high per-experiment costs of current methods and the inability of these methods to characterize materials having very small dimensions. Possible applications include bulk-processed materials with minimal dimensions, very scarce or hazardous materials, and materials that can only be made with microscale dimensions. Based on earlier work to develop laser-based techniques for detonating explosives, the current study examined the laser acceleration, or photonic driving, of small metal discs (''flyers'') that can generate controlled, planar shockwaves in test materials upon impact. Sub-nanosecond interferometric diagnostics were developed previously to examine the motion and impact of laser-driven flyers. To address a broad range of materials and stress states, photonic driving levels must be scaled up considerably from the levels used in earlier studies. Higher driving levels, however, increase concerns over laser-induced damage in optics and excessive heating of laser-accelerated materials. Sufficiently high levels require custom beam-shaping optics to ensure planar acceleration of flyers. The present study involved the development and evaluation of photonic driving systems at two driving levels, numerical simulations of flyer acceleration and impact using the CTH hydrodynamics code, design and fabrication of launch assemblies, improvements in diagnostic instrumentation, and validation experiments on both bulk and thin-film materials having well-established shock properties. The primary conclusion is that photonic driving techniques are viable additions to the methods currently used to obtain dynamic material properties. Improvements in launch conditions and diagnostics can certainly be made, but the main challenge to future applications will be the successful design and fabrication of test assemblies for materials of interest.
An increasing number of applications are requiring fiber transmission of high-intensity laser pulses. Our particular interests have led us to examine carefully the fiber transmission of Q-switched pulses from multimode Nd:YAG lasers at their fundamental wavelength. The maximum pulse energy that can be transmitted through a particular fiber is limited by the onset of laser-induced breakdown and damage mechanisms. Laser breakdown at the fiber entrance face is often the first limiting process to be encountered, but other mechanisms can result in catastrophic damage at either fiber face, within the initial `entry' segment of the fiber, and at other internal sites along the fiber path. In the course of our studies we have examined a number of factors that govern the relative importance of different mechanisms, including laser characteristics, the design and alignment of injection optics, fiber end-face preparation, and fiber routing. The present study emphasizes the important criteria for injection optics in high-intensity fiber transmission, and illustrates the opportunities that now exist for innovative designs of optics to meet these criteria. Our consideration of diffractive optics to achieve desired injection criteria began in 1993, and we have evaluated a progression of designs since that time. In the present study, two recent designs for injection optics are compared by testing a sufficient number of fibers with each design to establish statistics for the onset of laser-induced breakdown and damage. In this testing we attempted to hold constant other factors that can influence damage statistics. Both designs performed well, although one was less successful in meeting all injection criteria and consequently showed a susceptibility to a particular damage process.
In the present study, 10 impact tests were conducted on unpoled PZT 95/5, with 9% porosity and 2 at% Nb doping. These tests were instrumented to obtain time-resolved loading, unloading and span signatures. As well, PVDF gauges allowed shock timing to be established explicitly. The ferroelectric/antiferroelectric phases transition was manifested as a ramp to 0.4 GPa. The onset of crushup produced the most visible signature: a clear wave separation at 2.2 GPa followed by a highly dispersive wave. The end states also reflected crushup, and are consistent with earlier data and with related poled experiments. A span strength value of 0.17 GPa was measured for a shock stress of 0.5 GPa, this decreased to a very small value (no visible pullback signature) for a shock strength of 1.85 GPa.
Shock-induced depoling of the ferroelectric ceramic PZT 95/5 is utilized in a number of pulsed power devices. Several experimental and theoretical efforts are in progress in order to improve numerical simulations of these devices. In this study we have examined the shock response of normally poled PZT 95/5 under uniaxial strain conditions. On each experiment the current produced in an external circuit and the transmitted waveform at a window interface were recorded. The peak electrical field generated within the PZT sample was varied through the choice of external circuit resistance. Shock pressures were varied from 0.6 to 4.6 GPa, and peak electrical fields were varied from 0.2 to 37 kV/cm. For a 2.4 GPa shock and the lowest peak field, a nearly constant current governed simply by the remanent polarization and the shock velocity was recorded. Both decreasing the shock pressure and increasing the electrical field resulted in reduced current generation, indicating a retardation of the depoling kinetics.
Laser-induced damage mechanisms that can occur during high-intensity fiber transmission have been under study for a number of years. Our particular interest in laser initiation of explosives has led us to examine damage processes associated with the transmission of Q-switched, Nd:YAG pulses at 1.06 {micro}m through step-index, multimode, fused silica fiber. Laser breakdown at the fiber entrance face is often the first process to limit fiber transmission but catastrophic damage can also occur at either fiber end face, within the initial entry segment of the fiber, and at other internal sites along the fiber path. Past studies have examined how these various damage mechanisms depend upon fiber end-face preparation, fiber fixturing and routing, laser characteristics, and laser-to-fiber injection optics. In some applications of interest, however, a fiber transmission system may spend years in storage before it is used. Consequently, an important additional issue for these applications is whether or not there are aging processes that can result in lower damage thresholds over time. Fiber end-face contamination would certainly lower breakdown and damage thresholds at these surfaces, but careful design of hermetic seals in connectors and other end-face fixtures can minimize this possibility. A more subtle possibility would be a process for the slow growth of internal defects that could lead to lower thresholds for internal damage. In the current study, two approaches to stimulating the growth of internal defects were used in an attempt to produce observable changes in internal damage thresholds. In the first approach test fibers were subjected to a very high tensile stress for a time sufficient for some fraction to fail from static fatigue. In the second approach, test fibers were subjected to a combination of high tensile stress and large, cyclic temperature variations. Both of these approaches were rather arbitrary due to the lack of an established growth mechanism for internal defects. Damage characteristics obtained from fibers subjected to each of these aging environments were compared to results from fresh fibers tested under identical conditions. A surprising result was that internal damage was not observed in any of the tested fibers. Only breakdown at the fiber entrance face and catastrophic damage at both end faces were observed. Fiber end faces were not sealed during the accelerated aging environments, and thresholds at these faces were significantly lower in the aged fibers. However, most fibers transmitted relatively high pulse energies before damaging, and a large fraction never damaged before we reached the limits of our test laser. The absence of any observable affect on internal damage thresholds is encouraging, but the current results do not rule out the possibility that some other approach to accelerated aging could reveal a growth mechanism for internal defects.
Three methods for fiber end-face preparation based on the availability of exceptionally good cleaved surfaces from a commercial vendor were discussed. A few breakdown and damage processes were studied for this purpose. Results were also compared to previous measurements obtained from fibers which were mechanicallly polished using an optimized polishing. The mean values for maximum transmitted energy before breakdown or damage for the cleaved-only and cleaved-plus-flame polished fibers were a bit higher than the corresponding value for mechanical polished fibers.
Shock-induced depoling of the ferroelectric PZT 95/5 has been utilized in pulsed power applications for many years. Recently, new design and certification requirements have generated a strong interest in numerically simulating the operation of pulsed power devices. Because of a scarcity of relevant experimental data obtained within the past twenty years, we have initiated an extensive experimental study of the dynamic behavior of this material in support of simulation efforts. The experiments performed to date have been limited to examining the behavior of unpoled material. Samples of PZT 95/5 have been shocked to axial stresses from 0.5 to 5.0 GPa in planar impact experiments. Impact face conditions have been recorded using PVDF stress gauges, and transmitted wave profiles have been recorded either at window interfaces or at a free surface using laser interferometry (VISAR). The results significantly extend the stresses examined in prior studies of unpoled material, and ensure that a comprehensive experimental characterization of the mechanical behavior under shock loading is available for continuing development of PZT 95/5 material models.
Interest in the transmission of high intensities through optical fibers is being motivated by an increasing number of applications. Using different laser types and fiber materials, various studies are encountering transmission limitations due to laser-induced damage processes. The authors have found that fiber transmission is often limited by a plasma-forming breakdown occurring at the fiber entrance face. System attributes that will affect breakdown and damage thresholds include laser characteristics, the design and alignment of laser-to-fiber injection optics, and fiber end-face preparation. In the present work the authors have combined insights gained in past studies in order to establish what thresholds can be achieved if all system attributes can be optimized to some degree. The multimode laser utilized past modifications that produced a relatively smooth, quasi-Gaussian profile. The laser-to-fiber injection system achieved a relatively low value for the ratio of peak-to-average fluences at the fiber entrance face, incorporated a mode scrambler to generate a broad mode power distribution within the initial segment of the fiber path, and had improved fixturing to insure that the fiber axis was collinear with the incident laser beam. Fiber end faces were prepared by a careful mechanical polishing schedule followed by surface conditioning using a CO{sub 2} laser. In combination, these factors resulted in higher thresholds for breakdown and damage than they had achieved previously in studies that utilized a simple lens injection system.
Various applications are currently motivating interest in the transmission of very high laser intensities through optical fibers. As intensities within a fiber are increased, however, laser breakdown or laser-induced fiber damage will eventually occur and interrupt fiber transmission. For a number of years we have been studying these effects during the transmission of Q-switched, Nd/YAG laser pulses through step-index, multimode, fused-silica fiber. We have found that fiber transmission is often limited by a plasma-forming breakdown occurring at the fiber entrance face. This breakdown results in subtle surface modifications that can leave the surface more resistant to further breakdown or damage events. Catastrophic fiber damage can also occur as a result of a number of different mechanisms, with damage appearing at fiber end faces, within the initial ``entry`` segment of the fiber path, and at other internal sites due to effects related to the particular fiber routing. An overview of these past observations is presented, and issues requiring further study are identified.
A previous investigation of laser-induced damage mechanisms and corresponding thresholds in step-index, multimode fibers was motivated by an interest in optical systems for firing explosives. In the initial study, the output from a compact, multimode Nd/YAG laser was coupled into fiber cores of pure fused silica. End-face polishing steps were varied between successive fiber lots to produce improved finishes, and each fiber was subjected to a sequence of progressively increasing energy densities up to a value more than 80 J/cm{sup 2}. Essentially all of the tested fibers experienced a ``laser conditioning`` process at the front fiber face, in which a visible plasma was generated for one or more laser shots. Rather than produce progressive damage at the front surface, however, this process would eventually cease and leave the surface with improved damage resistance. Once past this conditioning process, the majority of fibers damaged at the rear end face. Other modes of damage were observed either at locations of fixturing stresses or at a location of high static tensile stress resulting from bends introduced to the fiber. The current experiments were conducted with a new laser having a shorter pulsewidth and a significantly different mode structure. The beam was injected into the fiber using a geometry that had been successful in the previous study in minimizing a damage mechanism which can occur at the core/cladding interface within the first few hundred fiber diameters. However, the different mode structure of the new laser apparently resulted in this mechanism dominating the current results.