Publications

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Nuclear power is an important and, the authors believe, essential component of a secure nuclear future. Although nuclear fuel cycles create materials that have some potential for use in nuclear weapons, with appropriate fuel cycles, nuclear power could reduce rather than increase real proliferation risk worldwide. Future fuel cycles could be designed to avoid plutonium production, generate minimal amounts of plutonium in proliferation-resistant amounts or configurations, and/or transparently and efficiently consume plutonium already created. Furthermore, a strong and viable US nuclear infrastructure, of which nuclear power is a large element, is essential if the US is to maintain a leadership or even participatory role in defining the global nuclear infrastructure and controlling the proliferation of nuclear weapons. By focusing on new fuel cycles and new reactor technologies, it is possible to advantageously burn and reduce nuclear materials that could be used for nuclear weapons rather than increase and/or dispose of these materials. Thus, the authors suggest that planners for a secure nuclear future use technology to design an ideal future. In this future, nuclear power creates large amounts of virtually atmospherically clean energy while significantly lowering the threat of proliferation through the thoughtful use, physical security, and agreed-upon transparency of nuclear materials. The authors must develop options for policy makers that bring them as close as practical to this ideal. Just as Atoms for Peace became the ideal for the first nuclear century, they see a potential nuclear future that contributes significantly to power for peace and prosperity.

This Executive Summary presents the methodology for determining containment requirements for spent-fuel transport casks under normal and hypothetical accident conditions. Three sources of radioactive material are considered: (1) the spent fuel itself, (2) radioactive material, referred to as CRUD, attached to the outside surfaces of fuel rod cladding, and (3) residual contamination adhering to interior surfaces of the cask cavity. The methodologies for determining the concentrations of freely suspended radioactive materials within a spent-fuel transport cask for these sources are discussed in much greater detail in three companion reports: ``A Method for Determining the Spent-Fuel Contribution to Transport Cask Containment Requirements,`` ``Estimate of CRUD Contribution to Shipping Cask Containment Requirements,`` and ``A Methodology for Estimating the Residual Contamination Contribution to the Source Term in a Spent-Fuel Transport Cask.`` Examples of cask containment requirements that combine the individually determined containment requirements for the three sources are provided, and conclusions from the three companion reports to this Executive Summary are presented.

This report examines containment requirements for spent-fuel transport containers that are transported under normal and hypothetical accident conditions. A methodology is described that estimates the probability of rod failure and the quantity of radioactive material released from breached rods. This methodology characterizes the dynamic environment of the cask and its contents and deterministically models the peak stresses that are induced in spent-fuel cladding by the mechanical and thermal dynamic environments. The peak stresses are evaluated in relation to probabilistic failure criteria for generated or preexisting ductile tearing and material fractures at cracks partially through the wall in fuel rods. Activity concentrations in the cask cavity are predicted from estimates of the fraction of gases, volatiles, and fuel fines that are released when the rod cladding is breached. Containment requirements based on the source term are calculated in terms of maximum permissible volumetric leak rates from the cask. Calculations are included for representative cask designs.

The Department of Energy`s (DOE`s) Office of Civilian Radioactive Waste Management (OCRWM) is in the process of developing a new generation of casks to transport spent fuel from commercial nuclear reactor facilities to federal waste facilities. In evaluating the needs of the cask development program a number of unresolved technical issues with potential impacts on the transportation system were identified. This paper provides three samples of issues being addressed by the Cask Systems Development Program for technical resolution: (1) burn-up credit, (2) containment source term evaluation, and (3) weeping.

The concept of allowing reactivity credit for the transmuted state of spent fuel offers both economic and risk incentives. This paper presents a general overview of the technical work being performed in support of the US Department of Energy (DOE) program to resolve issues related to the implementation of burnup credit. An analysis methodology is presented along with information representing the validation of the method against available experimental data. The experimental data that are applicable to burnup credit include chemical assay data for the validation of the isotopic prediction models, fresh fuel critical experiments for the validation of criticality calculations for various casks geometries, and reactor restart critical data to validate criticality calculations with spent fuel. The methodology has been specifically developed to be simple and generally applicable, therefore giving rise to uncertainties or sensitivities which are identified and quantified in terms of a percent bias in k{sub eff}. Implementation issues affecting licensing requirements and operational procedures are discussed briefly.

This report describes the ranges of the residual contamination that may build up in spent-fuel transport casks. These contamination ranges are calculated based on data taken from published reports and from previously unpublished data supplied by cask transporters. The data involve dose rate measurements, interior smear surveys, and analyses of water flushed out of cask cavities during decontamination operations. A methodology has been developed to estimate the effect of residual contamination on spent-fuel cask containment requirements. Factors in estimating the maximum permissible leak rates include the form of the residual contamination; possible release modes; internal gas-borne depletion; and the temperature, pressure, and vibration characteristics of the cask during transport under normal and accident conditions. 12 refs., 9 figs., 4 tabs.

The feasibility of performing, numerous spent fuel cask operations using fully integrated robotic systems is under evaluation. Using existing technology, operational and descriptive software and hardware in the form of robotic end effectors are being designed in conjunction with interfacing cask components. A robotic radiation and contamination survey system has been developed and used on mock-up cask hardware to evaluate the impact of such fully automated operations on cask design features and productivity. Based on experience gained from the survey system, numerous health physics operations can be reliably performed with little human intervention using a fully automated system. Such operations can also significantly reduce time requirements for cask-receiving operations. 7 refs., 51 figs., 6 tabs.

The Department of Energy sponsored a workshop on the use of burnup credit in the criticality design of spent fuel shipping casks on February 21 and 22, 1988. Twenty-five different presentations on many related topics were conducted, including the effects of burnup credit on the design and operation of spent fuel storage pools, casks and modules, and shipping casks; analysis and physics issues related to burnup credit; regulatory issues and criticality safety; economic incentives and risks associated with burnup credit; and methods for verifying spent fuel characteristics. An abbreviated version of the DOE workshop was repeated as a special session at the November 1988 American Nuclear Society Meeting in Washington, DC. Each of the invited speakers prepared detailed papers on his or her respective topic. The individual papers have been cataloged separately.

Spent pressurized-water reactor (PWR) and boiling-water reactor (BWR) fuel rods from three reactors were examined by hot cell periscope, energy dispersive x-ray analysis, and scanning electron micrography. In the case of fuel from the Quad Cities reactor, it was possible to develop a complete particle size distribution. It was found to be log-normal, with a median geometric diameter of 3 {mu}m and a standard deviation of 1.87 {mu}m. 5 refs., 5 figs., 1 tab.

Detailed models and analytical procedures are applied to the many complex aspects of spent fuel in transport including characterization of the fuel's irradiation conditions and initial states at the time of shipment, determination of the dynamic forces on the fuel assemblies that result from regulatory transportation accidents, modeling and analysis of the fuel's mechanical response to these forces, and estimation of the releasable radioactivity in the event of cladding breach. The methodology adopts a combined deterministic/probabilistic analysis approach in which each aspect of the problem is appropriately treated on the basis of its level of determinability. The results are obtained in the form of failure probabilities for each regulatory event considered. 3 refs., 6 figs.