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Location of the Monticello Mill Site.
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Background
The Monticello Mill Tailings Site is located in southeastern Utah, south of the town
of Monticello (see image to the right). The present climate at Monticello is
“sub-humid,” with an average annual precipitation of ~38 cm (15 inches) and an
average annual temperature of 7.8 ºC (46 ºF). In 1941, the Monticello mill was
constructed and used to process nearly a billion kilograms of ore. By 1960,
when operations were terminated, approximately 2 million cubic meters of
radioactive uranium mill tailings had been left behind from the operations. To
contain the mill tailings, DOE began construction of a repository south of the
original mill site in 1995, and in 1996 the construction of a composite double-
liner system at the base of the repository was completed.
The cover was designed to mitigate the release of radon gas to the surface and
to minimize water infiltration to the mill tailings. It consists of a thick
topsoil layer with vegetation that can store precipitation and allow evaporation
and transpiration via vegetation. This top layer overlies a coarse sand layer
that acts as a capillary barrier and is intended to drain any infiltrating water
laterally above a high-density polyethylene geomembrane. Beneath the geomembrane
is a compacted clay layer that serves as a barrier to radon gas transport and water
infiltration. The clay layer rests directly on top of the mill tailings. At the
base of the repository beneath the mill tailings is a double composite-liner
system composed of sand, two geomembrane liners, two geosynthetic clay-liners,
and a transmissive leachate collection system. The entire repository is surrounded
by Quaternary deposits consisting of sandy loam, clay, and pediment gravels.
Beneath the repository, two aquifers exist--a perched alluvial aquifer, as close
as several meters below the bottom of the repository and the regional Burro Canyon
aquifer beneath the alluvial aquifer. The perched aquifer was contaminated by mill
tailings prior to construction of the repository. The contaminants of concern
include uranium, as well as its radioactive decay products (thorium-230, radium-226,
radon-222), and heavy metals such as vanadium, lead-210, and arsenic. The Burro
Canyon aquifer and has not been contaminated. Between the alluvial aquifer and
the Burro Canyon aquifer are unsaturated layers of shale and sandstone. The
water from the upper alluvial aquifer is used for irrigation purposes, but all
drinking-water wells are located in the lower Burro Canyon aquifer.
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Monticello landfill cover and surrounding geology
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Objectives
The metrics and objectives used for the process assessment of the Monticello Mill Tailings
Repository case study are as follows:
- Percolation of water reaching mill tailings shall be less than 1x10-7 cm/s. This
is based on the prescribed maximum conductivity of the clay liner, where a unit-
gradient flow is assumed to equate percolation to conductivity.
- Average flux of radon-222 gas shall be less than 20 pCi/m2/s at the surface of the
repository cover.
- Combined radium-226 and radium-228 concentrations in groundwater shall be less than 5
pCi/L (only radium-226 is evaluated in this study).
- The effective dose to a member of the public from all pathways shall be less than 100
mrem/year (only radium-226 is evaluated in this study).
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Scenarios
The first step in the performance assessment is to develop relevant scenarios based on
performance objectives and applicable features, events, and processes at the site. For
a list of features, events, and processes at the site refer to section 4.1 of
SAND Report 2002-3131: Development of a Risk-Based
Probabilistic Performance-Assessment Method for Long-Term Cover Systems--2nd Edition
(Full reference).
A total of eight scenarios were chosen for this study:
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Conceptual Models
Once the scenarios were developed, conceptual models of the features, events, and
processes for each scenario could be formulated. The conceptual models include
contaminant source and release information, a description of transport mechanisms
and pathways, and a definition of modeling endpoints.
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The figure below shows the conceptual model for water percolation (scenarios
1 and 2) and gas transport (scenarios 3 and 4) through a composite (base-case)
cover design for present and future conditions. A 3% slope is assumed for the
drainage layer.
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The figure below shows the conceptual model for radionuclide transport
from the mill tailings to the shallow alluvial aquifer and location of receptor
well for present (scenario 5) and future (scenario 6)conditions.
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The figure below shows the conceptual model for radionuclide
transport from the mill tailings to the deep Burro Canyon aquifer and location
of receptor well for present (scenario 7) and future (scenario 8) conditions.
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Total-System Framework Models
The system used for this study was the
Framework for Risk Analysis in Multimedia Environmental Systems (FRAMES). FRAMES
was developed by Pacific Northwest National Laboratory (PNNL) with funding from DOE
and EPA. The FRAMES system provides a user-friendly platform for integrating medium
specific computer models, an extensive and editable contaminant database, a powerful
and flexible sensitivity/uncertainty module, and textual and graphical viewers for
presenting modeling outputs.scenarios 1 and 2 were simulated separately using HELP
v. 3.07 as a stand-alone code (Schroeder et al.,
1994). As part of this project,
HELP was integrated into FRAMES so that stochastic HELP simulations could be
performed from within the FRAMES architecture.
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Parameter Distribution for Process Models
Six process models, each with necessary input parameter distributions,
were included in the total-system model: (1) water percolation through the cover;
(2) radon gas trasport through the cover; (3) source-term release; (4) vadose-zone
transport; (5) saturated-zone transport; and (6) human exposure. For details on
parameter distributions for each of the process models, refer to section 4.3 of
SAND Report 2002-3131: Development of a Risk-Based
Probabilistic Performance-Assessment Method for Long-Term Cover Systems--2nd Edition
(Full reference).
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Results
Overall the results of this performance assessment illustrated how probabilistic
analyses could be used to evaluate long-term performance of covers against
regulatory metrics. The performance metrics can be risk-based, such as groundwater
concentration or dose, or they can be prescriptive metrics such as conductivity for
a particular layer of the cover. For detailed results, refer to section 4.4 of
SAND Report 2002-3131: Development of a Risk-Based
Probabilistic Performance-Assessment Method for Long-Term Cover Systems--2nd Edition
(Full reference). An example of the results follow.
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The following figure illustrates the cumulative probability distribution
of water percolation reaching the mill tailings for present and future
conditions (scenarios 1 and 2).
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The following figure illustrates the cumulative probability distribution
of simulated radon flux at the land surface for present and future conditions
(scenarios 3 and 4).
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The following figure illustrates the cumulative probability distribution
for peak Ra-226 concentration in the shallow alluvial aquifer for present and
future cond itions (scenarios 5-6). Note: concentration values of 0 are not
plotted on the log scale.
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The following figure illustrates the cumulative probability distribution
for peak cumulative dose for Ra-226 and its progeny from the shallow alluvial
aquifer for present and future conditions (scenarios 5-6). Note: dose values
of 0 are not plotted on the log scale.
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Alternative Designs
An alternative cover design was also evaluated for the Monticello disposal site using
probabilistic calculations. The performance of an
evapotranspiration (ET) cover was evaluated using the same probabilistic methods
described for the existing design. The ET cover consists of a simplified design
consisting of only the top layer. The ET cover concept makes use of the natural
moisture storage capacity of this upper layer of soil and the relatively high
efficiency of natural vegetation for the removal of moisture via evapotranspiration.
An assessment of landfill-cover cost versus performance can be made based on these
results.
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The following figure illustrates the cumulative probability distribution
of water percolation reaching the mill tailings for present and future
conditions (scenarios 1 and 2) and for the evapotranspiration cover. Although
the ET cover does not perform as well as the composite design with regard to
percolation flux, the vast majority of the realizations for future conditions
yield percolation flux values that are less than the regulatory limit. All of
the realizations for present conditions simulate a value of percolation flux
less than the regulatory limit. The expected behavior of the ET cover for
future conditions is percolation lower than the regulatory limit. In addition,
the ET cover is much cheaper to construct than similar designs such as the
one at Monticello (Dwyer, 2000).
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However, simulated Rn-222 flux through the surface of the landfill cover
is significantly higher for the ET cover relative to the composite cover, for
both present and future conditions, as shown in the figure below. A majority
of the realizations of the ET cover exceed the performance objective of 20
pCi/m2-s, for both present and future conditions. The 50th percentile values
of the simulated Rn-222 flux are about 25 pCi/m2-s and 30 pCi/m2-s for present
and future conditions, respectively. This result indicates an apparent
violation of the regulatory limits for radon flux with the ET cover design.
Thus, the ET cover design may be simplified, cheaper, and adequate for the
performance metrics of percolation flux, groundwater concentrations, and
cumulative dose, but inadequate to meet the radon flux standards.
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For detailed results, refer to section 4.5 of SAND
Report 2002-3131: Development of a Risk-Based Probabilistic Performance-Assessment
Method for Long-Term Cover Systems--2nd Edition
(Full reference).
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Sensitivity Analysis
A sensitivity analysis of the probabilistic assessment results can provide valuable
information regarding which components of the landfill cover system and which
parameters are most important to the simulated performance metric(s). This
information provides understanding about the relationship between uncertainty in
individual input parameters and the uncertainty in the performance of the system.
In addition, knowledge of the parameters having the greatest influence on future
performance can be used to help prioritize site characterization activities, to
help optimize landfill cover design, and to assist in the design of monitoring
systems. Using a sensitivity analysis provides the quantitative information
necessary to ensure that resources are directed to those aspects of the cover
system that “drive” performance and not on those aspects of cover design that
have little significance.
The following graph illustrates relative importance of stochastic input parameters
on the simulated peak cummulative dose.
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Summary and Conclusions
Overall the results of this performance assessment illustrated how probabilistic
analyses could be used to evaluate long-term performance of covers against
regulatory metrics. The performance metrics can be risk-based, such as groundwater
concentration or dose, or they can be prescriptive metrics such as conductivity
for a particular layer of the cover. In both cases, probabilistic performance
assessments can provide uncertainty and sensitivity analyses that identify the
parameters that are most important to long-term performance. These parameters may
be important for engineering design, environmental studies, and long-term
monitoring efforts to assist in prioritizing their efforts. In addition,
alternative designs for long-term covers can be evaluated using risk-based
performance metrics that are intended to protect human health and the environment.
These comparisons provide a more quantitative means to compare the performance of
cover designs while factoring in additional issues such as cost and schedule.
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